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Coherent Structural Dynamics and Electronic Correlations during an Ultrafast Insulator-to-Metal Phase Transition in VO2
Kübler, C., Ehrke, H., Huber, Rupert, Lopez, R., Halabica, A., Haglund Jr., R. F. und Leitenstorfer, A. (2007) Coherent Structural Dynamics and Electronic Correlations during an Ultrafast Insulator-to-Metal Phase Transition in VO2. Physical Review Letters (PRL) 99 (11), S. 116401.Veröffentlichungsdatum dieses Volltextes: 28 Jan 2011 07:20
Artikel
DOI zum Zitieren dieses Dokuments: 10.5283/epub.19123
Zusammenfassung
We directly trace the multi-THz conductivity of VO2 during an insulator-metal transition triggered by a 12-fs light pulse. The femtosecond dynamics of lattice and electronic degrees of freedom are spectrally discriminated. A coherent wave packet motion of V-V dimers at 6 THz modulates the lattice polarizability for approximately 1 ps. In contrast, the electronic conductivity settles to a constant ...
We directly trace the multi-THz conductivity of VO2 during an insulator-metal transition triggered by a 12-fs light pulse. The femtosecond dynamics of lattice and electronic degrees of freedom are spectrally discriminated. A coherent wave packet motion of V-V dimers at 6 THz modulates the lattice polarizability for approximately 1 ps. In contrast, the electronic conductivity settles to a constant value already after one V-V oscillation cycle. Based on our findings, we propose a qualitative model for the nonthermal phase transition.
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Details
| Dokumentenart | Artikel | ||||||||
| Titel eines Journals oder einer Zeitschrift | Physical Review Letters (PRL) | ||||||||
| Verlag: | American Physical Society | ||||||||
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| Band: | 99 | ||||||||
| Nummer des Zeitschriftenheftes oder des Kapitels: | 11 | ||||||||
| Seitenbereich: | S. 116401 | ||||||||
| Datum | 2007 | ||||||||
| Zusätzliche Informationen (Öffentlich) | » This publication has been selected for the Virtual Journal of Ultrafast Science » This publication has been selected for the Virtual Journal of Nanoscale Science and Technology | ||||||||
| Institutionen | Physik > Institut für Experimentelle und Angewandte Physik > Lehrstuhl Professor Huber > Arbeitsgruppe Rupert Huber | ||||||||
| Identifikationsnummer |
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| Klassifikation |
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| Dewey-Dezimal-Klassifikation | 500 Naturwissenschaften und Mathematik > 530 Physik | ||||||||
| Status | Veröffentlicht | ||||||||
| Begutachtet | Unbekannt / Keine Angabe | ||||||||
| An der Universität Regensburg entstanden | Unbekannt / Keine Angabe | ||||||||
| Dokumenten-ID | 19123 |
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