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Intrinsic lifetimes and anharmonic frequency shifts of long-wavelength optical phonons in polar crystals
Deinzer, Gernot
, Schmitt, Michael, Mayer, Andreas P. und Strauch, Dieter
(2004)
Intrinsic lifetimes and anharmonic frequency shifts of long-wavelength optical phonons in polar crystals.
Physical Review B 69, 014304.
Veröffentlichungsdatum dieses Volltextes: 05 Aug 2009 13:35
Artikel
DOI zum Zitieren dieses Dokuments: 10.5283/epub.1970
Zusammenfassung
Quantitative calculations of phonon lifetimes due to anharmonic three-phonon processes require knowledge of cubic anharmonic coupling coefficients. In order to determine the temperature dependence of phonon frequencies, anharmonic force constants of up to fourth order are needed. In polar crystals, the macroscopic electric field gives rise to nonanalytic terms in these coefficients. It is shown ...
Quantitative calculations of phonon lifetimes due to anharmonic three-phonon processes require knowledge of cubic anharmonic coupling coefficients. In order to determine the temperature dependence of phonon frequencies, anharmonic force constants of up to fourth order are needed. In polar crystals, the macroscopic electric field gives rise to nonanalytic terms in these coefficients. It is shown how these non-analytic terms can be determined from other physical quantities including higher-order dipole moments, Raman coefficients, and nonlinear susceptibilities. The contribution of these terms to the intrinsic damping of the long-wavelength optical phonon modes in GaAs has been determined by an ab initio calculation.
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| Dokumentenart | Artikel | ||||
| Titel eines Journals oder einer Zeitschrift | Physical Review B | ||||
| Verlag: | AMER PHYSICAL SOC | ||||
|---|---|---|---|---|---|
| Ort der Veröffentlichung: | COLLEGE PK | ||||
| Band: | 69 | ||||
| Seitenbereich: | 014304 | ||||
| Datum | 30 Januar 2004 | ||||
| Institutionen | Physik > Institut für Theoretische Physik > Entpflichtete oder im Ruhestand befindliche Professoren > Arbeitsgruppe Dieter Strauch | ||||
| Identifikationsnummer |
| ||||
| Stichwörter / Keywords | FUNCTIONAL PERTURBATION-THEORY; 2ND-ORDER RAMAN-SPECTRA; ABINITIO CALCULATION; QUANTUM WELLS; MONTE-CARLO; SEMICONDUCTORS; LINEWIDTH; | ||||
| Dewey-Dezimal-Klassifikation | 500 Naturwissenschaften und Mathematik > 530 Physik | ||||
| Status | Veröffentlicht | ||||
| Begutachtet | Ja, diese Version wurde begutachtet | ||||
| An der Universität Regensburg entstanden | Ja | ||||
| URN der UB Regensburg | urn:nbn:de:bvb:355-epub-19705 | ||||
| Dokumenten-ID | 1970 |
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