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Dynamics of Imidazolium Ionic Liquids from a Combined Dielectric Relaxation and Optical Kerr Effect Study: Evidence for Mesoscopic Aggregation

Turton, D. A. ; Hunger, J. ; Stoppa, A. ; Hefter, Glenn ; Thoman, A. ; Walther, M. ; Buchner, Richard ; Wynne, K.


The authors have measured the intermol. dynamics of the 1,3-dialkylimidazolium-based room-temp. ionic liqs. (RTILs) [emim][BF4], [emim][DCA], and [bmim][DCA] at 25 °C from <1 GHz to 10 THz by ultrafast optical Kerr effect (OKE) spectroscopy and dielec. relaxation spectroscopy (DRS) augmented by time-domain terahertz and far-IR FTIR spectroscopy. This concerted approach allows a more detailed ...


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