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Temporal Switching of Homo-FRET Pathways in Single-Chromophore Dimer Models of π-Conjugated Polymers

Stangl, Thomas ; Bange, Sebastian ; Schmitz, Daniela ; Würsch, Dominik ; Höger, Sigurd ; Vogelsang, Jan ; Lupton, John M.


A set of π-conjugated oligomer dimers templated in molecular scaffolds is presented as a model system for studying the interactions between chromophores in conjugated polymers (CPs). Single-molecule spectroscopy was used to reveal energy transfer dynamics between two oligomers in either a parallel or oblique-angle geometry. In particular, the conformation of single molecules embedded in a host ...


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