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Bottom-Up Self-Assembly of Amorphous Core-Shell-Shell Nanoparticles and Biomimetic Crystal Forms in Inorganic Silica-Carbonate Systems.

Eiblmeier, Josef ; Kellermeier, Matthias ; Deng, Mao ; Kienle, Lorenz ; Kunz, Werner


Silica-barium carbonate core-shell nanoparticles have been prepd. and characterized. At low silica concns., there was no evidence for an amorphous carbonate precursor phase and crystn. occurred immediately, resulting in elongated crystals that showed progressive self-similar branching due to the poisoning influence of silicate oligomers on the growth process. Above a certain threshold in the ...


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