Abstract
Phase-locked ultrashort pulses in the rich terahertz spectral range1, 2, 3, 4, 5, 6, 7, 8, 9, 10, 11, 12, 13, 14, 15, 16, 17, 18 have provided key insights into phenomena as diverse as quantum confinement7, first-order phase transitions8, 12, high-temperature superconductivity11 and carrier transport in nanomaterials1, 6, 13, 14, 15. Ultrabroadband electro-optic sampling of few-cycle field ...
Abstract
Phase-locked ultrashort pulses in the rich terahertz spectral range1, 2, 3, 4, 5, 6, 7, 8, 9, 10, 11, 12, 13, 14, 15, 16, 17, 18 have provided key insights into phenomena as diverse as quantum confinement7, first-order phase transitions8, 12, high-temperature superconductivity11 and carrier transport in nanomaterials1, 6, 13, 14, 15. Ultrabroadband electro-optic sampling of few-cycle field transients1 can even reveal novel dynamics that occur faster than a single oscillation cycle of light4, 8, 10. However, conventional terahertz spectroscopy is intrinsically restricted to ensemble measurements by the diffraction limit. As a result, it measures dielectric functions averaged over the size, structure, orientation and density of nanoparticles, nanocrystals or nanodomains. Here, we extend ultrabroadband time-resolved terahertz spectroscopy to the sub-nanoparticle scale (10 nm) by combining sub-cycle, field-resolved detection (10 fs) with scattering-type near-field scanning optical microscopy (s-NSOM)16, 17, 18, 19, 20, 21, 22, 23, 24, 25, 26. We trace the time-dependent dielectric function at the surface of a single photoexcited InAs nanowire in all three spatial dimensions and reveal the ultrafast (<50 fs) formation of a local carrier depletion layer.
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