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Eisele, Max ; Cocker, Tyler L. ; Huber, Markus A. ; Plankl, Markus ; Viti, L. ; Ercolani, D. ; Sorba, L. ; Vitiello, Miriam S. ; Huber, Rupert

Ultrafast multi-terahertz nano-spectroscopy with sub-cycle temporal resolution

Eisele, Max, Cocker, Tyler L., Huber, Markus A. , Plankl, Markus, Viti, L., Ercolani, D. , Sorba, L. , Vitiello, Miriam S. und Huber, Rupert (2014) Ultrafast multi-terahertz nano-spectroscopy with sub-cycle temporal resolution. Nature Photonics 8, S. 841-845.

Veröffentlichungsdatum dieses Volltextes: 02 Feb 2015 12:54
Artikel
DOI zum Zitieren dieses Dokuments: 10.5283/epub.31264


Zusammenfassung

Phase-locked ultrashort pulses in the rich terahertz spectral range(1-18) have provided key insights into phenomena as diverse as quantum confinement(7), first-order phase transitions(8,12), high-temperature superconductivity(11) and carrier transport in nanomaterials(1,6),(13-15). Ultrabroadband electrooptic sampling of few-cycle field transients(1) can even reveal novel dynamics that occur ...

Phase-locked ultrashort pulses in the rich terahertz spectral range(1-18) have provided key insights into phenomena as diverse as quantum confinement(7), first-order phase transitions(8,12), high-temperature superconductivity(11) and carrier transport in nanomaterials(1,6),(13-15). Ultrabroadband electrooptic sampling of few-cycle field transients(1) can even reveal novel dynamics that occur faster than a single oscillation cycle of light(4,8,10). However, conventional terahertz spectroscopy is intrinsically restricted to ensemble measurements by the diffraction limit. As a result, it measures dielectric functions averaged over the size, structure, orientation and density of nanoparticles, nanocrystals or nanodomains. Here, we extend ultrabroadband time-resolved terahertz spectroscopy to the sub-nanoparticle scale (10 nm) by combining subcycle, field-resolved detection (10 fs) with scattering-type near-field scanning optical microscopy (s-NSOM)(16-26). We trace the time-dependent dielectric function at the surface of a single photoexcited InAs nanowire in all three spatial dimensions and reveal the ultrafast (<50 fs) formation of a local carrier depletion layer.



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Details

DokumentenartArtikel
Titel eines Journals oder einer ZeitschriftNature Photonics
Verlag:NATURE PUBLISHING GROUP
Ort der Veröffentlichung:LONDON
Band:8
Seitenbereich:S. 841-845
Datum5 Oktober 2014
InstitutionenPhysik > Institut für Experimentelle und Angewandte Physik > Lehrstuhl Professor Huber > Arbeitsgruppe Rupert Huber
Identifikationsnummer
WertTyp
10.1038/NPHOTON.2014.225DOI
Stichwörter / KeywordsNANOWIRES; MATTER; LIGHT;
Dewey-Dezimal-Klassifikation500 Naturwissenschaften und Mathematik > 530 Physik
StatusVeröffentlicht
BegutachtetJa, diese Version wurde begutachtet
An der Universität Regensburg entstandenJa
Dokumenten-ID31264

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