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Ultrafast multi-terahertz nano-spectroscopy with sub-cycle temporal resolution
Eisele, Max, Cocker, Tyler L., Huber, Markus A.
, Plankl, Markus, Viti, L., Ercolani, D.
, Sorba, L.
, Vitiello, Miriam S. und Huber, Rupert
(2014)
Ultrafast multi-terahertz nano-spectroscopy with sub-cycle temporal resolution.
Nature Photonics 8, S. 841-845.
Veröffentlichungsdatum dieses Volltextes: 02 Feb 2015 12:54
Artikel
DOI zum Zitieren dieses Dokuments: 10.5283/epub.31264
Zusammenfassung
Phase-locked ultrashort pulses in the rich terahertz spectral range(1-18) have provided key insights into phenomena as diverse as quantum confinement(7), first-order phase transitions(8,12), high-temperature superconductivity(11) and carrier transport in nanomaterials(1,6),(13-15). Ultrabroadband electrooptic sampling of few-cycle field transients(1) can even reveal novel dynamics that occur ...
Phase-locked ultrashort pulses in the rich terahertz spectral range(1-18) have provided key insights into phenomena as diverse as quantum confinement(7), first-order phase transitions(8,12), high-temperature superconductivity(11) and carrier transport in nanomaterials(1,6),(13-15). Ultrabroadband electrooptic sampling of few-cycle field transients(1) can even reveal novel dynamics that occur faster than a single oscillation cycle of light(4,8,10). However, conventional terahertz spectroscopy is intrinsically restricted to ensemble measurements by the diffraction limit. As a result, it measures dielectric functions averaged over the size, structure, orientation and density of nanoparticles, nanocrystals or nanodomains. Here, we extend ultrabroadband time-resolved terahertz spectroscopy to the sub-nanoparticle scale (10 nm) by combining subcycle, field-resolved detection (10 fs) with scattering-type near-field scanning optical microscopy (s-NSOM)(16-26). We trace the time-dependent dielectric function at the surface of a single photoexcited InAs nanowire in all three spatial dimensions and reveal the ultrafast (<50 fs) formation of a local carrier depletion layer.
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Details
| Dokumentenart | Artikel | ||||
| Titel eines Journals oder einer Zeitschrift | Nature Photonics | ||||
| Verlag: | NATURE PUBLISHING GROUP | ||||
|---|---|---|---|---|---|
| Ort der Veröffentlichung: | LONDON | ||||
| Band: | 8 | ||||
| Seitenbereich: | S. 841-845 | ||||
| Datum | 5 Oktober 2014 | ||||
| Institutionen | Physik > Institut für Experimentelle und Angewandte Physik > Lehrstuhl Professor Huber > Arbeitsgruppe Rupert Huber | ||||
| Identifikationsnummer |
| ||||
| Stichwörter / Keywords | NANOWIRES; MATTER; LIGHT; | ||||
| Dewey-Dezimal-Klassifikation | 500 Naturwissenschaften und Mathematik > 530 Physik | ||||
| Status | Veröffentlicht | ||||
| Begutachtet | Ja, diese Version wurde begutachtet | ||||
| An der Universität Regensburg entstanden | Ja | ||||
| Dokumenten-ID | 31264 |
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