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Periodic Charging of Individual Molecules Coupled to the Motion of an Atomic Force Microscopy Tip.

Kocić, Nemanja ; Weiderer, Peter ; Keller, Stephan ; Decurtins, Silvio ; Liu, Shi-Xia ; Repp, Jascha


Individual molecules at the edges of self-assembled islands grown on Ag(111) can be deliberately switched in their charge state with the electric field from a scanning-probe tip. Close to the threshold voltage for a charge state transition, periodic switching of the charge is directly driven by the cantilever motion in frequency-modulated atomic force microscopy (AFM), as can be deduced from the ...


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