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Haug, Tobias ; Klemm, Philippe ; Bange, Sebastian ; Lupton, John M.

Hot-electron intraband luminescence from single hot spots in noble-metal nanoparticle films

Article

Haug, Tobias, Klemm, Philippe, Bange, Sebastian and Lupton, John M. (2015) Hot-electron intraband luminescence from single hot spots in noble-metal nanoparticle films. Physical Review Letters (PRL). (In Press)

DOI to cite this document: 10.5283/epub.32147


Abstract

Disordered noble-metal nanoparticle films exhibit highly localized and stable non-linear light emission from sub-diffraction regions upon illumination by near-infrared femtosecond pulses. Such hot spot emission spans a continuum in the visible and near-infrared spectral range. Strong plasmonic enhancement of light-matter interaction and the resulting complexity of experimental observations have ...

Disordered noble-metal nanoparticle films exhibit highly localized and stable non-linear light emission from sub-diffraction regions upon illumination by near-infrared femtosecond pulses. Such hot spot emission spans a continuum in the visible and near-infrared spectral range. Strong plasmonic enhancement of light-matter interaction and the resulting complexity of experimental observations have prevented the development of a universal understanding of the origin of light emission. Here, we study the dependence of emission spectra on excitation irradiance and provide the most direct evidence yet that the continuum emission observed from both silver and gold nanoparticle aggregate surfaces is caused by recombination of hot electrons within the conduction band. The electron gas in the emiting particles, which is effectively decoupled from the lattice temperature for the duration of emission, reaches effective temperatures of several thousand Kelvin and acts as a sub-diffraction incandescent light source on sub-picosecond time scales.


Involved Institutions


Details

Item typeArticle
Journal or Publication TitlePhysical Review Letters (PRL)
PublisherAmerican Physical Society
Open Access TypeDue to SHERPA/RoMEO
Date2015
Date of publication14 Jul 2015 09:08
InstitutionsPhysics > Institute of Experimental and Applied Physics > Chair Professor Lupton > Group John Lupton
Dewey Decimal Classification500 Science > 530 Physics
StatusIn Press
RefereedYes, this version has been refereed
Created at the University of RegensburgYes
URN of the UB Regensburgurn:nbn:de:bvb:355-epub-321473
Item ID32147

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