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No photocatalyst required – versatile, visible light mediated transformations with polyhalomethanes

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Franz, Johannes F. ; Kraus, Wolfgang B. ; Zeitler, Kirsten
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Date of publication of this fulltext: 19 Feb 2016 14:18


A visible light mediated, but photocatalyst-free method for the oxidative α-CH functionalization of tertiary amines with a broad scope of carbon- and heteroatom nucleophiles using polyhalomethanes has been developed. In addition, the pivotal visible light triggered activation of polyhalomethanes offers mild conditions for efficient Kharasch-type additions onto non-activated olefins. Preliminary mechanistic studies are reported.

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