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Control of Reactivity and Regioselectivity for On-Surface Dehydrogenative Aryl-Aryl Bond Formation.

Kocić, Nemanja ; Liu, Xunshan ; Chen, Songjie ; Decurtins, Silvio ; Krejčí, Ondřej ; Jelinek, Pavel ; Repp, Jascha ; Liu, Shi-Xia



Abstract

Regioselectivity is of fundamental importance in chemical synthesis. Although many concepts for site-selective reactions are well established for solution chemistry, it is not a priori clear whether they can easily be transferred to reactions taking place on a metal surface. A metal will fix the chemical potential of the electrons and perturb the electronic states of the reactants because of ...

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