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Conformational control of benzophenone-sensitized charge transfer in dinucleotides

URN to cite this document:
urn:nbn:de:bvb:355-epub-342296
DOI to cite this document:
10.5283/epub.34229
Merz, Thomas ; Wenninger, M. ; Weinberger, Michael ; Riedle, E. ; Wagenknecht, Hans-Achim ; Schütz, Martin
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Date of publication of this fulltext: 04 Aug 2016 11:04


Abstract

Charge transfer in DNA cannot be understood without addressing the complex conformational flexibility, which occurs on a wide range of timescales. In order to reduce this complexity four dinucleotide models 1X consisting of benzophenone linked by a phosphodiester to one of the natural nucleosides X = A, G, T, C were studied in water and methanol. The theoretical work focuses on the dynamics and ...

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