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Tracking the ultrafast motion of a single molecule by femtosecond orbital imaging

Cocker, Tyler L. ; Peller, Dominik ; Yu, Ping ; Repp, Jascha ; Huber, Rupert


Watching a single molecule move on its intrinsic timescale has been one of the central goals of modern nanoscience, and calls for measurements that combine ultrafast temporal resolution(1-8) with atomic spatial resolution(9-30). Steady-state experiments access the requisite spatial scales, as illustrated by direct imaging of individual molecular orbitals using scanning tunnelling microscopy(9-11) ...


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