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Effect of Conjugation Pathway in Metal-Free Room-Temperature Dual Singlet–Triplet Emitters for Organic Light-Emitting Diodes

Ratzke, Wolfram ; Schmitt, Lisa ; Matsuoka, Hideto ; Bannwarth, Christoph ; Retegan, Marius ; Bange, Sebastian ; Klemm, Philippe ; Neese, Frank ; Grimme, Stefan ; Schiemann, Olav ; Lupton, John M.


Metal-free dual singlettriplet organic light-emitting diode (OLED) emitters can provide direct insight into spin statistics, spin correlations and spin relaxation phenomena, through a comparison of fluorescence to phosphorescence intensity. Remarkably, such materials can also function at room temperature, exhibiting phosphorescence lifetimes of several milliseconds. Using electroluminescence, ...


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