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Lanthanide Ions Coupled with Photoinduced Electron Transfer
Generate Strong Reduction Potentials from Visible Light

Meyer, Andreas Uwe , Slanina, Tomas , Heckel, Alexander and König, Burkhard (2017) Lanthanide Ions Coupled with Photoinduced Electron Transfer
Generate Strong Reduction Potentials from Visible Light.
Chemistry - A European Journal 23, pp. 7900-7904.

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Abstract

Metal ions can have beneficial effects on photoinduced electron transfer. Merging such metal-ion-coupled electron transfer (MCET) with consecutive photoinduced electron transfer (conPET) enables the one-electron reduction of chlorobenzene with blue light in the presence of diisopropylethylamine as an electron donor. The presence of the metal ions extends the substrate scope of the photoredox catalysis to extreme reduction potentials (beyond - 3 V vs. SCE).


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Item type:Article
Date:2017
Institutions:Chemistry and Pharmacy > Institut für Organische Chemie > Lehrstuhl Prof. Dr. Burkhard König
Projects:GRK 1626 Chemische Photokatalyse
Identification Number:
ValueType
10.1002/chem.201701665DOI
Keywords:ORGANIC-SYNTHESIS; SAMARIUM DIIODIDE; PHOTOREDOX CATALYSIS; ARYL HALIDES; CARBONYL-COMPOUNDS; ALKYL-HALIDES; FLAVIN ANALOG; EOSIN Y; IODIDE; COMPLEXES; aryl radical; C-C bond formation; lanthanides; photoredox catalysis; photoreduction
Dewey Decimal Classification:500 Science > 540 Chemistry & allied sciences
Status:Published
Refereed:Yes, this version has been refereed
Created at the University of Regensburg:Partially
Item ID:35599
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