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Teaching old compounds new tricks: DDQ-Photocatalyzed C-H
Amination of Arenes with Carbamates, Urea and N-Heterocycles

Das, Somnath, Natarajan, Palani and König, Burkhard (2017) Teaching old compounds new tricks: DDQ-Photocatalyzed C-H
Amination of Arenes with Carbamates, Urea and N-Heterocycles.
Chemistry - A European Journal 23, pp. 18161-18165.

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Abstract

The C-H amination of benzene derivatives was achieved using DDQ as photocatalyst and BocNH(2) as the amine source under aerobic conditions and visible light irradiation. Electron-deficient and electron-rich benzenes react as substrates with moderate to good product yields. The amine scope of the reaction comprises Boc-amine, carbamates, pyrazoles, sulfonimides and urea. Preliminary mechanistic ...

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Item type:Article
Date:2017
Institutions:Chemistry and Pharmacy > Institut für Organische Chemie > Lehrstuhl Prof. Dr. Burkhard König
Projects:GRK 1626 Chemische Photokatalyse
Identification Number:
ValueType
10.1002/chem.201705442DOI
Keywords:LATE-STAGE FUNCTIONALIZATION; CROSS-COUPLING REACTIONS; ORGANIC PHOTOREDOX CATALYSIS; MEDICINAL CHEMISTS TOOLBOX; CHARGE-TRANSFER COMPLEXES; ELECTRON-TRANSFER; EXCITED-STATE; DRUG DESIGN; LIGHT; BENZENE; C-H amination; charge-transfer complexes; electron-deficient arenes; heterocycles; photocatalysis
Dewey Decimal Classification:500 Science > 540 Chemistry & allied sciences
Status:Published
Refereed:Yes, this version has been refereed
Created at the University of Regensburg:Yes
Item ID:36366
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