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Dielectric Engineering of Electronic Correlations in a van der Waals Heterostructure
Steinleitner, Philipp, Merkl, Philipp, Graf, Alexander, Nagler, Philipp, Watanabe, Kenji
, Taniguchi, Takashi, Zipfel, Jonas, Schüller, Christian, Korn, Tobias
, Chernikov, Alexey, Brem, Samuel, Selig, Malte, Berghäuser, Gunnar, Malic, Ermin und Huber, Rupert
(2018)
Dielectric Engineering of Electronic Correlations in a van der Waals Heterostructure.
Nano Letters 18 (2), S. 1402-1409.
Veröffentlichungsdatum dieses Volltextes: 14 Feb 2018 15:33
Artikel
DOI zum Zitieren dieses Dokuments: 10.5283/epub.36719
Zusammenfassung
Heterostructures of van der Waals bonded layered materials offer unique means to tailor dielectric screening with atomic-layer precision, opening a fertile field of fundamental research. The optical analyses used so far have relied on interband spectroscopy. Here we demonstrate how a capping layer of hexagonal boron nitride (hBN) renormalizes the internal structure of excitons in a WSe2 monolayer ...
Heterostructures of van der Waals bonded layered materials offer unique means to tailor dielectric screening with atomic-layer precision, opening a fertile field of fundamental research. The optical analyses used so far have relied on interband spectroscopy. Here we demonstrate how a capping layer of hexagonal boron nitride (hBN) renormalizes the internal structure of excitons in a WSe2 monolayer using intraband transitions. Ultrabroadband terahertz probes sensitively map out the full complex-valued mid-infrared conductivity of the heterostructure after optical injection of is A excitons. This approach allows us to trace the energies and line widths of the atom-like 1s-2p transition of optically bright and dark excitons as well as the densities of these quasiparticles. The excitonic resonance red shifts and narrows in the WSe2/hBN heterostructure compared to the bare monolayer. Furthermore, the ultrafast temporal evolution of the mid-infrared response function evidences the formation of optically dark excitons from an initial bright population. Our results provide key insight into the effect of nonlocal screening on electron hole correlations and open new possibilities of dielectric engineering of van der Waals heterostructures.
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Steinleitner, Philipp, Merkl, Philipp, Graf, Alexander, Nagler, Philipp, Watanabe, KenjiVorschau
, Taniguchi, Takashi, Zipfel, Jonas, Schüller, Christian, Korn, Tobias
, Chernikov, Alexey, Brem, Samuel, Selig, Malte, Berghäuser, Gunnar, Malic, Ermin und Huber, Rupert
(2018)
Dielectric Engineering of Electronic Correlations in a van der Waals Heterostructure.
Nano Letters 18 (2), S. 1402-1409.
[Gegenwärtig angezeigt]-
Steinleitner, Philipp
, Merkl, Philipp, Graf, Alexander, Nagler, Philipp, Wantanabe, Kenji, Taniguchi, Takashi, Zipfel, Jonas, Schüller, Christian
, Korn, Tobias
, Chernikov, Alexey, Huber, Rupert
, Brem, Samuel
, Selig, Malte, Berghäuser, Gunnar und Malic, Ermin
(2018)
Data archive of "Dielectric engineering of electronic correlations in a van der Waals heterostructure".
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Details
| Dokumentenart | Artikel | ||||
| Titel eines Journals oder einer Zeitschrift | Nano Letters | ||||
| Verlag: | AMER CHEMICAL SOC | ||||
|---|---|---|---|---|---|
| Ort der Veröffentlichung: | WASHINGTON | ||||
| Band: | 18 | ||||
| Nummer des Zeitschriftenheftes oder des Kapitels: | 2 | ||||
| Seitenbereich: | S. 1402-1409 | ||||
| Datum | 24 Januar 2018 | ||||
| Institutionen | Physik > Institut für Experimentelle und Angewandte Physik > Lehrstuhl Professor Huber > Arbeitsgruppe Rupert Huber Physik > Institut für Experimentelle und Angewandte Physik > Lehrstuhl Professor Lupton > Arbeitsgruppe Christian Schüller | ||||
| Identifikationsnummer |
| ||||
| Stichwörter / Keywords | METAL DICHALCOGENIDE HETEROSTRUCTURES; LIGHT-EMITTING-DIODES; P-N-JUNCTIONS; MONOLAYER WSE2; 2-DIMENSIONAL MATERIALS; SEMICONDUCTOR; SPECTROSCOPY; EXCITONS; MOS2/WS2; LAYER; Dichalcogenides; atomically thin 2D crystals; van der Waals heterostructures; dielectric engineering; dark excitons | ||||
| Dewey-Dezimal-Klassifikation | 500 Naturwissenschaften und Mathematik > 530 Physik | ||||
| Status | Veröffentlicht | ||||
| Begutachtet | Ja, diese Version wurde begutachtet | ||||
| An der Universität Regensburg entstanden | Ja | ||||
| URN der UB Regensburg | urn:nbn:de:bvb:355-epub-367191 | ||||
| Dokumenten-ID | 36719 |
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