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Reorganization energy upon charging a single molecule on an insulator measured by atomic force microscopy

Fatayer, Shadi ; Schuler, Bruno ; Steurer, Wolfram ; Scivetti, Ivan ; Repp, Jascha ; Gross, Leo ; Persson, Mats ; Meyer, Gerhard



Abstract

Intermolecular single-electron transfer on electrically insulating films is a key process in molecular electronics1,2,3,4 and an important example of a redox reaction5,6. Electron-transfer rates in molecular systems depend on a few fundamental parameters, such as interadsorbate distance, temperature and, in particular, the Marcus reorganization energy7. This crucial parameter is the energy gain ...

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