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Time-Domain Interferometry of Surface Plasmons at Nonlinear Continuum Hot Spots in Films of Silver Nanoparticles
Klemm, Philippe, Haug, Tobias, Bange, Sebastian
und Lupton, John M.
(2014)
Time-Domain Interferometry of Surface Plasmons at Nonlinear Continuum Hot Spots in Films of Silver Nanoparticles.
Physical Review Letters 113 (266805).
Veröffentlichungsdatum dieses Volltextes: 14 Mrz 2019 08:24
Artikel
DOI zum Zitieren dieses Dokuments: 10.5283/epub.38433
Zusammenfassung
Nonlinear continuum generation from diffraction-limited hot spots in rough silver films exhibits striking narrow-band intensity resonances in excitation wavelength. Time-domain Fourier spectroscopy uncovers how these resonances arise due to the formation of a "plasmon staircase", a discreteness in the fundamental oscillation of the plasmon excitations responsible for generating the white-light ...
Nonlinear continuum generation from diffraction-limited hot spots in rough silver films exhibits striking narrow-band intensity resonances in excitation wavelength. Time-domain Fourier spectroscopy uncovers how these resonances arise due to the formation of a "plasmon staircase", a discreteness in the fundamental oscillation of the plasmon excitations responsible for generating the white-light continuum. Whereas multiple scattering from discrete antennas can be invoked to explain hot spot formation in random assemblies of isolated particles, hot spots in films of fused nanoparticles are excited by interfering propagating surface plasmons, launched by scattering from individual nanoparticle antennas. For closed films, discrete propagating plasmons interact coherently over distances of tens of microns to pump the hot spot.
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| Dokumentenart | Artikel | ||||||
| Titel eines Journals oder einer Zeitschrift | Physical Review Letters | ||||||
| Verlag: | AMER PHYSICAL SOC | ||||||
|---|---|---|---|---|---|---|---|
| Ort der Veröffentlichung: | COLLEGE PK | ||||||
| Band: | 113 | ||||||
| Nummer des Zeitschriftenheftes oder des Kapitels: | 266805 | ||||||
| Datum | 2014 | ||||||
| Institutionen | Physik > Institut für Experimentelle und Angewandte Physik > Lehrstuhl Professor Lupton > Arbeitsgruppe John Lupton | ||||||
| Identifikationsnummer |
| ||||||
| Stichwörter / Keywords | ENHANCED RAMAN-SCATTERING; NOBLE-METALS; LIGHT; GENERATION; INTERFERENCE; MICROSCOPY; EXCITATION; DYNAMICS; | ||||||
| Dewey-Dezimal-Klassifikation | 500 Naturwissenschaften und Mathematik > 530 Physik | ||||||
| Status | Veröffentlicht | ||||||
| Begutachtet | Ja, diese Version wurde begutachtet | ||||||
| An der Universität Regensburg entstanden | Ja | ||||||
| URN der UB Regensburg | urn:nbn:de:bvb:355-epub-384332 | ||||||
| Dokumenten-ID | 38433 |
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