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Molecular Water Lilies: Orienting Single Molecules in a Polymer Film by Solvent Vapor Annealing

Würsch, Dominik ; Hofmann, Felix J. ; Eder, Theresa ; Aggarwal, Vikas A. ; Idelson, Alissa ; Höger, Sigurd ; Lupton, John M. ; Vogelsang, Jan


The microscopic orientation and position of photoactive molecules is crucial to the operation of optoelectronic devices such as OLEDs and solar cells. Here, we introduce a shape-persistent macrocyclic molecule as an excellent fluorescent probe to simply measure (i) its orientation by rotating the excitation polarization and recording the strength of modulation in photoluminescence (PL) and (ii) ...


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