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Zipfel, Jonas ; Holler, Johannes ; Mitioglu, Anatolie A. ; Ballottin, Mariana V. ; Nagler, Philipp ; Stier, Andreas V. ; Taniguchi, Takashi ; Watanabe, Kenji ; Crooker, Scott A. ; Christianen, Peter C. M. ; Korn, Tobias ; Chernikov, Alexey

Spatial extent of the excited exciton states in WS2 monolayers from diamagnetic shifts

Zipfel, Jonas, Holler, Johannes, Mitioglu, Anatolie A., Ballottin, Mariana V., Nagler, Philipp, Stier, Andreas V., Taniguchi, Takashi, Watanabe, Kenji, Crooker, Scott A., Christianen, Peter C. M., Korn, Tobias and Chernikov, Alexey (2018) Spatial extent of the excited exciton states in WS2 monolayers from diamagnetic shifts. Physical Review B 98 (7), 075438.

Date of publication of this fulltext: 18 Jul 2019 11:59
Article
DOI to cite this document: 10.5283/epub.40520


Abstract

We experimentally study the radii of excitons in hBN-encapsulated WS(2 )monolayers by means of magneto-optical reflectance spectroscopy at cryogenic temperatures in magnetic fields up to 29 T. We observe field-induced energy shifts of the exciton ground and excited states due to valley Zeeman and diamagnetic effects. We find the g factor of the first excited state of -4.2 +/- 0.1 to be ...

We experimentally study the radii of excitons in hBN-encapsulated WS(2 )monolayers by means of magneto-optical reflectance spectroscopy at cryogenic temperatures in magnetic fields up to 29 T. We observe field-induced energy shifts of the exciton ground and excited states due to valley Zeeman and diamagnetic effects. We find the g factor of the first excited state of -4.2 +/- 0.1 to be essentially equal to that of the ground state of -4.35 +/- 0.1. From diamagnetic shifts, we determine the root mean square radii of the excitons. The radius of the first excited state is found to be 5-8 nm and that of the ground state around 2 nm Our results further confirm the Wannier-Mott nature of the exciton quasiparticles in monolayer semiconductors and the assignment of the optical resonances in absorption-type measurements. They also provide additional support for the applicability of the effective mass hydrogenlike models in these systems.



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Details

Item typeArticle
Journal or Publication TitlePhysical Review B
Publisher:AMER PHYSICAL SOC
Open Access Type:Due to SHERPA/RoMEO
Place of Publication:COLLEGE PK
Volume:98
Number of Issue or Book Chapter:7
Page Range:075438
Date2018
InstitutionsPhysics > Institute of Experimental and Applied Physics > Chair Professor Huber > Group Rupert Huber
Identification Number
ValueType
10.1103/PhysRevB.98.075438DOI
KeywordsSEMICONDUCTOR; WSE2; SPECTRA; ENERGY; MOS2;
Dewey Decimal Classification500 Science > 530 Physics
StatusPublished
RefereedYes, this version has been refereed
Created at the University of RegensburgYes
URN of the UB Regensburgurn:nbn:de:bvb:355-epub-405207
Item ID40520

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