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Spatial extent of the excited exciton states in WS2 monolayers from diamagnetic shifts
Zipfel, Jonas, Holler, Johannes, Mitioglu, Anatolie A., Ballottin, Mariana V., Nagler, Philipp, Stier, Andreas V., Taniguchi, Takashi, Watanabe, Kenji, Crooker, Scott A., Christianen, Peter C. M., Korn, Tobias
and Chernikov, Alexey
(2018)
Spatial extent of the excited exciton states in WS2 monolayers from diamagnetic shifts.
Physical Review B 98 (7), 075438.
Date of publication of this fulltext: 18 Jul 2019 11:59
Article
DOI to cite this document: 10.5283/epub.40520
Abstract
We experimentally study the radii of excitons in hBN-encapsulated WS(2 )monolayers by means of magneto-optical reflectance spectroscopy at cryogenic temperatures in magnetic fields up to 29 T. We observe field-induced energy shifts of the exciton ground and excited states due to valley Zeeman and diamagnetic effects. We find the g factor of the first excited state of -4.2 +/- 0.1 to be ...
We experimentally study the radii of excitons in hBN-encapsulated WS(2 )monolayers by means of magneto-optical reflectance spectroscopy at cryogenic temperatures in magnetic fields up to 29 T. We observe field-induced energy shifts of the exciton ground and excited states due to valley Zeeman and diamagnetic effects. We find the g factor of the first excited state of -4.2 +/- 0.1 to be essentially equal to that of the ground state of -4.35 +/- 0.1. From diamagnetic shifts, we determine the root mean square radii of the excitons. The radius of the first excited state is found to be 5-8 nm and that of the ground state around 2 nm Our results further confirm the Wannier-Mott nature of the exciton quasiparticles in monolayer semiconductors and the assignment of the optical resonances in absorption-type measurements. They also provide additional support for the applicability of the effective mass hydrogenlike models in these systems.
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| Item type | Article | ||||
| Journal or Publication Title | Physical Review B | ||||
| Publisher: | AMER PHYSICAL SOC | ||||
|---|---|---|---|---|---|
| Open Access Type: | Due to SHERPA/RoMEO | ||||
| Place of Publication: | COLLEGE PK | ||||
| Volume: | 98 | ||||
| Number of Issue or Book Chapter: | 7 | ||||
| Page Range: | 075438 | ||||
| Date | 2018 | ||||
| Institutions | Physics > Institute of Experimental and Applied Physics > Chair Professor Huber > Group Rupert Huber | ||||
| Identification Number |
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| Keywords | SEMICONDUCTOR; WSE2; SPECTRA; ENERGY; MOS2; | ||||
| Dewey Decimal Classification | 500 Science > 530 Physics | ||||
| Status | Published | ||||
| Refereed | Yes, this version has been refereed | ||||
| Created at the University of Regensburg | Yes | ||||
| URN of the UB Regensburg | urn:nbn:de:bvb:355-epub-405207 | ||||
| Item ID | 40520 |
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