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DNA-catalyzed Henry Reaction in Pure Water and the Striking Influence of Organic Buffer Systems

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Häring, Marleen ; Pérez-Madrigal, Maria M. ; Kühbeck, Dennis ; Pettignano, Asja ; Quignard, Françoise ; Diaz Diaz, David
License: Creative Commons Attribution 4.0
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Date of publication of this fulltext: 12 Feb 2020 13:14


In this manuscript we report a critical evaluation of the ability of natural DNA to mediate the nitroaldol (Henry) reaction at physiological temperature in pure water. Under these conditions, no background reaction took place (i.e., control experiment without DNA). Both heteroaromatic aldehydes (e.g., 2-pyridinecarboxaldehyde) and aromatic aldehydes bearing strong or moderate electron-withdrawing ...


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