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Deazaflavin reductive photocatalysis involves excited semiquinone radicals

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Graml, Andreas ; Neveselý, Tomáš ; Kutta, Roger Jan ; Cibulka, Radek ; König, Burkhard
License: Creative Commons Attribution 4.0
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Date of publication of this fulltext: 02 Jul 2020 04:57


Flavin-mediated photocatalytic oxidations are established in synthetic chemistry. In contrast, their use in reductive chemistry is rare. Deazaflavins with a much lower reduction potential are even better suited for reductive chemistry rendering also deazaflavin semiquinones as strong reductants. However, no direct evidence exists for the involvement of these radical species in reductive ...


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