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Holler, Johannes ; Meier, Sebastian ; Kempf, Michael ; Nagler, Philipp ; Watanabe, Kenji ; Taniguchi, Takashi ; Korn, Tobias ; Schüller, Christian

Low-frequency Raman scattering in WSe2−MoSe2 heterobilayers: Evidence for atomic reconstruction

Holler, Johannes, Meier, Sebastian, Kempf, Michael, Nagler, Philipp, Watanabe, Kenji , Taniguchi, Takashi, Korn, Tobias und Schüller, Christian (2020) Low-frequency Raman scattering in WSe2−MoSe2 heterobilayers: Evidence for atomic reconstruction. Applied Physics Letters 117, 013104.

Veröffentlichungsdatum dieses Volltextes: 21 Jul 2020 05:56
Artikel
DOI zum Zitieren dieses Dokuments: 10.5283/epub.43491


Zusammenfassung

We investigate WSe2-MoSe2 heterobilayers with different twist angles theta +/- delta between the two layers by low-frequency Raman scattering. In sufficiently aligned samples with theta = 0 degrees or theta = 60 degrees and delta less than or similar to 3 degrees, we observe an interlayer shear mode (ISM), which is a clear sign of a commensurate bilayer structure, i.e., the layers must undergo an ...

We investigate WSe2-MoSe2 heterobilayers with different twist angles theta +/- delta between the two layers by low-frequency Raman scattering. In sufficiently aligned samples with theta = 0 degrees or theta = 60 degrees and delta less than or similar to 3 degrees, we observe an interlayer shear mode (ISM), which is a clear sign of a commensurate bilayer structure, i.e., the layers must undergo an atomic reconstruction to form R-type or H-type stacking orders. We find slightly different ISM energies of about 18cm(-1) and 17cm(-1) for H-type and R-type reconstructions, respectively, independent of the exact value of theta +/- delta. Our findings are corroborated by the fact that the ISM is not observed in samples with twist angles, which deviate by delta > 3 degrees from 0 degrees or 60 degrees. This is expected since, in such incommensurate structures, with the possibility of Moire-lattice formation, there is no restoring force for an ISM. Furthermore, we observe the ISM even in sufficiently aligned heterobilayers, which are encapsulated in hexagonal Boron nitride. This is particularly relevant for the characterization of high-quality heterostructure devices.



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    Vorschau
    Holler, Johannes, Meier, Sebastian, Kempf, Michael, Nagler, Philipp, Watanabe, Kenji , Taniguchi, Takashi, Korn, Tobias und Schüller, Christian (2020) Low-frequency Raman scattering in WSe2−MoSe2 heterobilayers: Evidence for atomic reconstruction. Applied Physics Letters 117, 013104. [Gegenwärtig angezeigt]

Details

DokumentenartArtikel
Titel eines Journals oder einer ZeitschriftApplied Physics Letters
Verlag:AMER INST PHYSICS
Ort der Veröffentlichung:MELVILLE
Band:117
Seitenbereich:013104
Datum8 Juli 2020
InstitutionenPhysik > Institut für Experimentelle und Angewandte Physik
Identifikationsnummer
WertTyp
10.1063/5.0012249DOI
Stichwörter / KeywordsDER-WAALS HETEROSTRUCTURES; MONOLAYER; EXCITONS; STACKING;
Dewey-Dezimal-Klassifikation500 Naturwissenschaften und Mathematik > 530 Physik
StatusVeröffentlicht
BegutachtetJa, diese Version wurde begutachtet
An der Universität Regensburg entstandenJa
URN der UB Regensburgurn:nbn:de:bvb:355-epub-434915
Dokumenten-ID43491

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