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Low-frequency Raman scattering in WSe2−MoSe2 heterobilayers: Evidence for atomic reconstruction
Holler, Johannes, Meier, Sebastian, Kempf, Michael, Nagler, Philipp, Watanabe, Kenji
, Taniguchi, Takashi, Korn, Tobias
und Schüller, Christian
(2020)
Low-frequency Raman scattering in WSe2−MoSe2 heterobilayers: Evidence for atomic reconstruction.
Applied Physics Letters 117, 013104.
Veröffentlichungsdatum dieses Volltextes: 21 Jul 2020 05:56
Artikel
DOI zum Zitieren dieses Dokuments: 10.5283/epub.43491
Zusammenfassung
We investigate WSe2-MoSe2 heterobilayers with different twist angles theta +/- delta between the two layers by low-frequency Raman scattering. In sufficiently aligned samples with theta = 0 degrees or theta = 60 degrees and delta less than or similar to 3 degrees, we observe an interlayer shear mode (ISM), which is a clear sign of a commensurate bilayer structure, i.e., the layers must undergo an ...
We investigate WSe2-MoSe2 heterobilayers with different twist angles theta +/- delta between the two layers by low-frequency Raman scattering. In sufficiently aligned samples with theta = 0 degrees or theta = 60 degrees and delta less than or similar to 3 degrees, we observe an interlayer shear mode (ISM), which is a clear sign of a commensurate bilayer structure, i.e., the layers must undergo an atomic reconstruction to form R-type or H-type stacking orders. We find slightly different ISM energies of about 18cm(-1) and 17cm(-1) for H-type and R-type reconstructions, respectively, independent of the exact value of theta +/- delta. Our findings are corroborated by the fact that the ISM is not observed in samples with twist angles, which deviate by delta > 3 degrees from 0 degrees or 60 degrees. This is expected since, in such incommensurate structures, with the possibility of Moire-lattice formation, there is no restoring force for an ISM. Furthermore, we observe the ISM even in sufficiently aligned heterobilayers, which are encapsulated in hexagonal Boron nitride. This is particularly relevant for the characterization of high-quality heterostructure devices.
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Holler, Johannes, Meier, Sebastian, Kempf, Michael, Nagler, Philipp, Watanabe, KenjiVorschau
, Taniguchi, Takashi, Korn, Tobias
und Schüller, Christian
(2020)
Low-frequency Raman scattering in WSe2−MoSe2 heterobilayers: Evidence for atomic reconstruction.
Applied Physics Letters 117, 013104.
[Gegenwärtig angezeigt]-
Holler, Johannes
, Meier, Sebastian, Kempf, Michael, Nagler, Philipp, Watanabe, Kenji
, Taniguchi, Takashi, Korn, Tobias
und Schüller, Christian
(2021)
Data archive of "Low-frequency Raman scattering in WSe2−MoSe2 heterobilayers: Evidence for atomic reconstruction".
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Details
| Dokumentenart | Artikel | ||||
| Titel eines Journals oder einer Zeitschrift | Applied Physics Letters | ||||
| Verlag: | AMER INST PHYSICS | ||||
|---|---|---|---|---|---|
| Ort der Veröffentlichung: | MELVILLE | ||||
| Band: | 117 | ||||
| Seitenbereich: | 013104 | ||||
| Datum | 8 Juli 2020 | ||||
| Institutionen | Physik > Institut für Experimentelle und Angewandte Physik | ||||
| Identifikationsnummer |
| ||||
| Stichwörter / Keywords | DER-WAALS HETEROSTRUCTURES; MONOLAYER; EXCITONS; STACKING; | ||||
| Dewey-Dezimal-Klassifikation | 500 Naturwissenschaften und Mathematik > 530 Physik | ||||
| Status | Veröffentlicht | ||||
| Begutachtet | Ja, diese Version wurde begutachtet | ||||
| An der Universität Regensburg entstanden | Ja | ||||
| URN der UB Regensburg | urn:nbn:de:bvb:355-epub-434915 | ||||
| Dokumenten-ID | 43491 |
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