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Sub-cycle atomic-scale forces coherently control a single-molecule switch

Peller, Dominik ; Kastner, Lukas Z. ; Buchner, Thomas ; Roelcke, Carmen ; Albrecht, Florian ; Moll, Nikolaj ; Huber, Rupert ; Repp, Jascha


Scanning probe techniques can leverage atomically precise forces to sculpt matter at surfaces, atom by atom. These forces have been applied quasi-statically to create surface structures1--7 and influence chemical processes8,9, but exploiting local dynamics10--14 to realize coherent control on the atomic scale remains an intriguing prospect. Chemical reactions15--17, conformational changes18,19 ...


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