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Dynamic Quenching of Triplet Excitons in Single Conjugated Polymer Chains

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Schedlbauer, Jakob ; Scherf, Ullrich ; Vogelsang, Jan ; Lupton, John M.
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Date of publication of this fulltext: 08 Oct 2020 08:07


By measuring the fluorescence photon statistics of single chains of a conjugated polymer, we determine the lifetime of the metastable dark state, the triplet exciton. The single molecule emits single photons one at a time, giving rise to photon antibunching. These photons appear bunched in time over longer time scales because of excursions to the triplet dark state. Remarkably, this triplet ...


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