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Plankl, Markus ; Faria Junior, Paulo E. ; Mooshammer, Fabian ; Siday, Tom ; Zizlsperger, Martin ; Sandner, Fabian ; Schiegl, Felix ; Maier, Simon ; Huber, Markus A. ; Gmitra, Martin ; Fabian, Jaroslav ; Boland, Jessica L. ; Cocker, Tyler L. ; Huber, Rupert

Subcycle contact-free nanoscopy of ultrafast interlayer transport in atomically thin heterostructures

Plankl, Markus, Faria Junior, Paulo E., Mooshammer, Fabian , Siday, Tom, Zizlsperger, Martin, Sandner, Fabian, Schiegl, Felix, Maier, Simon , Huber, Markus A. , Gmitra, Martin, Fabian, Jaroslav , Boland, Jessica L. , Cocker, Tyler L. and Huber, Rupert (2021) Subcycle contact-free nanoscopy of ultrafast interlayer transport in atomically thin heterostructures. Nature Photonics 15, pp. 594-600.

Date of publication of this fulltext: 21 May 2021 04:36
Article
DOI to cite this document: 10.5283/epub.45829


Abstract

Tunnelling is one of the most fundamental manifestations of quantum mechanics. The recent advent of lightwave-driven scanning tunnelling microscopy has revolutionized ultrafast nanoscience by directly resolving electron tunnelling in electrically conducting samples on the relevant ultrashort length- and timescales. Here, we introduce a complementary approach based on terahertz near-field ...

Tunnelling is one of the most fundamental manifestations of quantum mechanics. The recent advent of lightwave-driven scanning tunnelling microscopy has revolutionized ultrafast nanoscience by directly resolving electron tunnelling in electrically conducting samples on the relevant ultrashort length- and timescales. Here, we introduce a complementary approach based on terahertz near-field microscopy to perform ultrafast nano-videography of tunnelling processes even in insulators. The central idea is to probe the evolution of the local polarizability of electron-hole pairs with evanescent terahertz fields, which we detect with subcycle temporal resolution. In a proof of concept, we resolve femtosecond interlayer transport in van der Waals heterobilayers and reveal pronounced variations of the local formation and annihilation of interlayer excitons on deeply subwavelength, nanometre scales. Such contact-free nanoscopy of tunnelling-induced dynamics should be universally applicable to conducting and non-conducting samples and reveal how ultrafast transport processes shape functionalities in a wide range of condensed matter systems. Subcycle nano-videography of charge-transfer dynamics in WSe2/WS2 heterostructures is obtained by using a terahertz near-field microscopy. The central idea is to probe the local polarizability of electron-hole pairs with evanescent terahertz fields.



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  • [img] Plankl, Markus, Faria Junior, Paulo E., Mooshammer, Fabian , Siday, Tom, Zizlsperger, Martin, Sandner, Fabian, Schiegl, Felix, Maier, Simon , Huber, Markus A. , Gmitra, Martin, Fabian, Jaroslav , Boland, Jessica L. , Cocker, Tyler L. and Huber, Rupert (2021) Subcycle contact-free nanoscopy of ultrafast interlayer transport in atomically thin heterostructures. Nature Photonics 15, pp. 594-600. [Currently displayed]

Details

Item typeArticle
Journal or Publication TitleNature Photonics
Publisher:Nature
Open Access Type:No Open Access
Place of Publication:BERLIN
Volume:15
Page Range:pp. 594-600
Date13 May 2021
InstitutionsPhysics > Institute of Theroretical Physics > Chair Professor Richter > Group Jaroslav Fabian
Physics > Institute of Experimental and Applied Physics > Chair Professor Huber > Group Rupert Huber
Identification Number
ValueType
10.1038/s41566-021-00813-yDOI
KeywordsSINGLE-MOLECULE; TERAHERTZ; SPECTROSCOPY; POLARITONS; MICROSCOPY; DYNAMICS
Dewey Decimal Classification500 Science > 530 Physics
StatusPublished
RefereedYes, this version has been refereed
Created at the University of RegensburgYes
URN of the UB Regensburgurn:nbn:de:bvb:355-epub-458297
Item ID45829

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