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Lin, Kai‐Qiang ; Holler, Johannes ; Bauer, Jonas M. ; Parzefall, Philipp ; Scheuck, Marten ; Peng, Bo ; Korn, Tobias ; Bange, Sebastian ; Lupton, John M. ; Schüller, Christian

Large‐Scale Mapping of Moiré Superlattices by Hyperspectral Raman Imaging

Lin, Kai‐Qiang , Holler, Johannes , Bauer, Jonas M., Parzefall, Philipp , Scheuck, Marten, Peng, Bo, Korn, Tobias, Bange, Sebastian, Lupton, John M. und Schüller, Christian (2021) Large‐Scale Mapping of Moiré Superlattices by Hyperspectral Raman Imaging. Advanced Materials 33, S. 2008333.

Veröffentlichungsdatum dieses Volltextes: 13 Jul 2021 04:42
Artikel
DOI zum Zitieren dieses Dokuments: 10.5283/epub.46326


Zusammenfassung

Moire superlattices can induce correlated-electronic phases in twisted van der Waals materials: strongly correlated quantum phenomena emerge, such as superconductivity and the Mott-insulating state. However, moire superlattices produced through artificial stacking can be quite inhomogeneous, which hampers the development of a clear correlation between the moire period and the emerging electrical ...

Moire superlattices can induce correlated-electronic phases in twisted van der Waals materials: strongly correlated quantum phenomena emerge, such as superconductivity and the Mott-insulating state. However, moire superlattices produced through artificial stacking can be quite inhomogeneous, which hampers the development of a clear correlation between the moire period and the emerging electrical and optical properties. Here, it is demonstrated in twisted-bilayer transition-metal dichalcogenides that low-frequency Raman scattering can be utilized not only to detect atomic reconstruction, but also to map out the inhomogeneity of the moire lattice over large areas. The method is established based on the finding that both the interlayer-breathing mode and moire phonons are highly susceptible to the moire period and provide characteristic fingerprints. Hyperspectral Raman imaging visualizes microscopic domains of a 5 degrees twisted-bilayer sample with an effective twist-angle resolution of about 0.1 degrees. This ambient methodology can be conveniently implemented to characterize and preselect high-quality areas of samples for subsequent device fabrication, and for transport and optical experiments.



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Details

DokumentenartArtikel
Titel eines Journals oder einer ZeitschriftAdvanced Materials
Verlag:Wiley
Ort der Veröffentlichung:WEINHEIM
Band:33
Seitenbereich:S. 2008333
Datum9 Juli 2021
InstitutionenPhysik > Institut für Experimentelle und Angewandte Physik > Lehrstuhl Professor Lupton > Arbeitsgruppe Christian Schüller
Physik > Institut für Experimentelle und Angewandte Physik > Lehrstuhl Professor Lupton > Arbeitsgruppe John Lupton
Projekte
Gefördert von: Deutsche Forschungsgemeinschaft (DFG) (443378379)
Gefördert von: Deutsche Forschungsgemeinschaft (DFG) (443361515)
Identifikationsnummer
WertTyp
10.1002/adma.202008333DOI
Stichwörter / KeywordsGRAPHENE; MULTILAYER; MODES; SHEAR; SCATTERING; INTERFACE; MOS2; hyperspectral Raman imaging; interlayer breathing modes; low-frequency Raman scattering; moire phonons; moire superlattices
Dewey-Dezimal-Klassifikation500 Naturwissenschaften und Mathematik > 530 Physik
StatusVeröffentlicht
BegutachtetJa, diese Version wurde begutachtet
An der Universität Regensburg entstandenZum Teil
URN der UB Regensburgurn:nbn:de:bvb:355-epub-463269
Dokumenten-ID46326

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