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How Lattice and Charge Fluctuations Control Carrier Dynamics in Halide Perovskites

Mayers, Matthew Z. ; Tan, Liang Z. ; Egger, David A. ; Rappe, Andrew M. ; Reichman, David R.


Here we develop a microscopic approach aimed at the description of a suite of physical effects related to carrier transport in, and the optical properties of, halide perovskites. Our theory is based on the description of the nuclear dynamics to all orders and goes beyond the common assumption of linear electron-phonon coupling in describing the carrier dynamics and band gap characteristics. When ...


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