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Synthesis and Characterization of the First Tin Fluoride Borate Sn3 [B3 O7 ]F with Second Harmonic Generation Response

Schönegger, Sandra ; Jantz, Stephan G. ; Saxer, Andreas ; Bayarjargal, Lkhamsuren ; Winkler, Björn ; Pielnhofer, Florian ; Höppe, Henning A. ; Huppertz, Hubert


The new non-centrosymmetric tin fluoride borate Sn-3[B3O7]F was synthesized hydrothermally, and was characterized by single-crystal and powder X-ray diffraction, vibrational spectroscopy, DFT calculations, second harmonic generation (SHG) measurements, thermogravimetry, and differential scanning calorimetry. Its SHG response is about 12 times that of quartz. The compound crystallizes in the ...


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