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Revealing weak spin-orbit coupling effects on charge carriers in a π -conjugated polymer

Malissa, H. ; Miller, R. ; Baird, D. L. ; Jamali, S. ; Joshi, G. ; Bursch, M. ; Grimme, S. ; van Tol, J. ; Lupton, J. M. ; Boehme, C.


We measure electrically detected magnetic resonance on organic light-emitting diodes made of the polymer poly[2-methoxy-5-(2-ethylhexyloxy)-1,4-phenylenevinylene] at room temperature and high magnetic fields where spectral broadening of the resonance due to spin-orbit coupling (SOC) exceeds that due to the local hyperfine fields. Density-functional-theory calculations on an open-shell model of ...


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