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Directing energy transfer in Pt(bodipy)(mercaptopyrene) dyads

Irmler, Peter ; Gogesch, Franciska S. ; Mang, André ; Bodensteiner, Michael ; Larsen, Christopher B. ; Wenger, Oliver S. ; Winter, Rainer F.



Abstract

We report on the photophysical properties of three dyads that combine a 4,4-difluoro-4-bora-3a,4a-diaza-s-indacene (bodipy, BDP) and a mercaptopyrene (SPyr) dye ligand at a Pt(PEt3)(2) fragment. sigma-Bonding of the dyes to the Pt ion promotes intersystem crossing (ISC) via the external heavy atom effect. The coupling of efficient ISC with charge-transfer from the electron-rich mercaptopyrene to ...

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