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Nanoscale force sensing of an ultrafast nonlinear optical response

Schumacher, Zeno ; Rejali, Rasa ; Pachlatko, Raphael ; Spielhofer, Andreas ; Nagler, Philipp ; Miyahara, Yoichi ; Cooke, David G. ; Grütter, Peter



Abstract

The nonlinear optical response of a material is a sensitive probe of electronic and structural dynamics under strong light fields. The induced microscopic polarizations are usually detected via their far-field light emission, thus limiting spatial resolution. Several powerful near-field techniques circumvent this limitation by employing local nanoscale scatterers; however, their signal strength ...

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