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Tuning Deazaflavins Towards Highly Potent Reducing Photocatalysts Guided by Mechanistic Understanding – Enhancement of the Key Step by the Internal Heavy Atom Effect

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Pavlovska, Tetiana ; Král Lesný, David ; Svobodová, Eva ; Hoskovcová, Irena ; Archipowa, Nataliya ; Kutta, Roger Jan ; Cibulka, Radek
Date of publication of this fulltext: 30 Aug 2022 05:36

This publication is part of the DEAL contract with Wiley.


Deazaflavins are well suited for reductive chemistry acting via a consecutive photo-induced electron transfer, in which their triplet state and semiquinone - the latter is formed from the former after electron transfer from a sacrificial electron donor - are key intermediates. Guided by mechanistic investigations aiming to increase intersystem crossing by the internal heavy atom effect and ...


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