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Electrostatic and Environmental Control of the Trion Fine Structure in Transition Metal Dichalcogenide Monolayers
Zhumagulov, Yaroslav V.
, Vagov, Alexei, Gulevich, Dmitry R.
und Perebeinos, Vasili
(2022)
Electrostatic and Environmental Control of the Trion Fine Structure in Transition Metal Dichalcogenide Monolayers.
Nanomaterials 12 (21), S. 3728.
Veröffentlichungsdatum dieses Volltextes: 04 Nov 2022 14:32
Artikel
DOI zum Zitieren dieses Dokuments: 10.5283/epub.53123
Zusammenfassung
Charged excitons or trions are essential for optical spectra in low-dimensional doped monolayers (ML) of transitional metal dichalcogenides (TMDC). Using a direct diagonalization of the three-body Hamiltonian, we calculate the low-lying trion states in four types of TMDC MLs as a function of doping and dielectric environment. We show that the fine structure of the trion is the result of the ...
Charged excitons or trions are essential for optical spectra in low-dimensional doped monolayers (ML) of transitional metal dichalcogenides (TMDC). Using a direct diagonalization of the three-body Hamiltonian, we calculate the low-lying trion states in four types of TMDC MLs as a function of doping and dielectric environment. We show that the fine structure of the trion is the result of the interplay between the spin-valley fine structure of the single-particle bands and the exchange interaction. We demonstrate that by variations of the doping and dielectric environment, the fine structure of the trion energy can be tuned, leading to anticrossing of the bright and dark states, with substantial implications for the optical spectra of the TMDC ML.
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Details
| Dokumentenart | Artikel | ||||
| Titel eines Journals oder einer Zeitschrift | Nanomaterials | ||||
| Verlag: | MDPI | ||||
|---|---|---|---|---|---|
| Ort der Veröffentlichung: | BASEL | ||||
| Band: | 12 | ||||
| Nummer des Zeitschriftenheftes oder des Kapitels: | 21 | ||||
| Seitenbereich: | S. 3728 | ||||
| Datum | 24 Oktober 2022 | ||||
| Institutionen | Physik > Institut für Theoretische Physik | ||||
| Identifikationsnummer |
| ||||
| Stichwörter / Keywords | PHOTOLUMINESCENCE; BIEXCITONS; excitons; trions; transition metal dichalcogenides | ||||
| Dewey-Dezimal-Klassifikation | 500 Naturwissenschaften und Mathematik > 530 Physik | ||||
| Status | Veröffentlicht | ||||
| Begutachtet | Ja, diese Version wurde begutachtet | ||||
| An der Universität Regensburg entstanden | Ja | ||||
| URN der UB Regensburg | urn:nbn:de:bvb:355-epub-531238 | ||||
| Dokumenten-ID | 53123 |
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