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Zhumagulov, Yaroslav V. ; Vagov, Alexei ; Gulevich, Dmitry R. ; Perebeinos, Vasili

Electrostatic and Environmental Control of the Trion Fine Structure in Transition Metal Dichalcogenide Monolayers

Artikel

Zhumagulov, Yaroslav V. , Vagov, Alexei, Gulevich, Dmitry R. und Perebeinos, Vasili (2022) Electrostatic and Environmental Control of the Trion Fine Structure in Transition Metal Dichalcogenide Monolayers. Nanomaterials 12 (21), S. 3728.

DOI zum Zitieren dieses Dokuments: 10.5283/epub.53123


Zusammenfassung

Charged excitons or trions are essential for optical spectra in low-dimensional doped monolayers (ML) of transitional metal dichalcogenides (TMDC). Using a direct diagonalization of the three-body Hamiltonian, we calculate the low-lying trion states in four types of TMDC MLs as a function of doping and dielectric environment. We show that the fine structure of the trion is the result of the ...

Charged excitons or trions are essential for optical spectra in low-dimensional doped monolayers (ML) of transitional metal dichalcogenides (TMDC). Using a direct diagonalization of the three-body Hamiltonian, we calculate the low-lying trion states in four types of TMDC MLs as a function of doping and dielectric environment. We show that the fine structure of the trion is the result of the interplay between the spin-valley fine structure of the single-particle bands and the exchange interaction. We demonstrate that by variations of the doping and dielectric environment, the fine structure of the trion energy can be tuned, leading to anticrossing of the bright and dark states, with substantial implications for the optical spectra of the TMDC ML.



Beteiligte Einrichtungen


Details

DokumentenartArtikel
Titel eines Journals oder einer ZeitschriftNanomaterials
VerlagMDPI
Open Access ArtGold (mit APC - nicht UR)
Ort der VeröffentlichungBASEL
Band12
Nummer des Zeitschriftenheftes oder des Kapitels21
SeitenbereichS. 3728
Datum24 Oktober 2022
Veröffentlichungsdatum04 Nov 2022 14:32
InstitutionenPhysik > Institut für Theoretische Physik
Identifikationsnummer
WertTyp
10.3390/nano12213728DOI
Stichwörter / KeywordsPHOTOLUMINESCENCE; BIEXCITONS; excitons; trions; transition metal dichalcogenides
Dewey-Dezimal-Klassifikation500 Naturwissenschaften und Mathematik > 530 Physik
StatusVeröffentlicht
BegutachtetJa, diese Version wurde begutachtet
An der Universität Regensburg entstandenJa
URN der UB Regensburgurn:nbn:de:bvb:355-epub-531238
Dokumenten-ID53123

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