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Ultrafast Nanoscopy of High-Density Exciton Phases in WSe2
Siday, Tom
, Sandner, Fabian, Brem, Samuel, Zizlsperger, Martin, Perea-Causín, Raül, Schiegl, Felix, Nerreter, Svenja, Plankl, Markus, Merkl, Philipp, Mooshammer, Fabian
, Huber, Markus A.
, Malic, Ermin und Huber, Rupert
(2022)
Ultrafast Nanoscopy of High-Density Exciton Phases in WSe2.
Nano Letters 22, S. 2561-2568.
Veröffentlichungsdatum dieses Volltextes: 14 Nov 2022 09:47
Artikel
DOI zum Zitieren dieses Dokuments: 10.5283/epub.53190
Zusammenfassung
The density-driven transition of an exciton gas into an electron- hole plasma remains a compelling question in condensed matter physics. In two-dimensional transition metal dichalcogenides, strongly bound excitons can undergo this phase change after transient injection of electron-hole pairs. Unfortunately, unavoidable nanoscale inhomogeneity in these materials has impeded quantitative ...
The density-driven transition of an exciton gas into an electron- hole plasma remains a compelling question in condensed matter physics. In two-dimensional transition metal dichalcogenides, strongly bound excitons can undergo this phase change after transient injection of electron-hole pairs. Unfortunately, unavoidable nanoscale inhomogeneity in these materials has impeded quantitative investigation into this elusive transition. Here, we demonstrate how ultrafast polarization nanoscopy can capture the Mott transition through the density-dependent recombination dynamics of electron-hole pairs within a WSe2 homobilayer. For increasing carrier density, an initial monomolecular recombination of optically dark excitons transitions continuously into a bimolecular recombination of an unbound electron-hole plasma above 7 x 10(12) cm(-2). We resolve how the Mott transition modulates over nanometer length scales, directly evidencing the strong inhomogeneity in stacked monolayers. Our results demonstrate how ultrafast polarization nanoscopy could unveil the interplay of strong electronic correlations and interlayer coupling within a diverse range of stacked and twisted two-dimensional materials.
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Siday, Tom
, Sandner, Fabian, Brem, Samuel, Zizlsperger, Martin, Perea-Causín, Raül, Schiegl, Felix, Nerreter, Svenja, Plankl, Markus, Merkl, Philipp, Mooshammer, Fabian
, Huber, Markus A.
, Malic, Ermin und Huber, Rupert
(2022)
Ultrafast Nanoscopy of High-Density Exciton Phases in WSe2.
Nano Letters 22, S. 2561-2568.
[Gegenwärtig angezeigt]-
Siday, Tom
, Sandner, Fabian, Brem, Samuel
, Zizlsperger, Martin
, Perea-Causin, Raul, Schiegl, Felix
, Nerreter, Svenja
, Plankl, Markus, Merkl, Philipp, Mooshammer, Fabian
, Huber, Markus A.
, Malic, Ermin und Huber, Rupert
(2022)
Data archive of 'Ultrafast Nanoscopy of High-Density Exciton Phases in WSe_2' in Nano Letters 22, 2561 (2022).
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Details
| Dokumentenart | Artikel | ||||
| Titel eines Journals oder einer Zeitschrift | Nano Letters | ||||
| Verlag: | AMER CHEMICAL SOC | ||||
|---|---|---|---|---|---|
| Ort der Veröffentlichung: | WASHINGTON | ||||
| Band: | 22 | ||||
| Seitenbereich: | S. 2561-2568 | ||||
| Datum | 14 Februar 2022 | ||||
| Institutionen | Physik > Institut für Experimentelle und Angewandte Physik > Lehrstuhl Professor Huber > Arbeitsgruppe Rupert Huber | ||||
| Identifikationsnummer |
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| Stichwörter / Keywords | MONOLAYER; Mott transition; exciton; ultrafast dynamics; near-field microscopy; terahertz; transition metal dichalcogenides | ||||
| Dewey-Dezimal-Klassifikation | 500 Naturwissenschaften und Mathematik > 530 Physik | ||||
| Status | Veröffentlicht | ||||
| Begutachtet | Ja, diese Version wurde begutachtet | ||||
| An der Universität Regensburg entstanden | Ja | ||||
| URN der UB Regensburg | urn:nbn:de:bvb:355-epub-531902 | ||||
| Dokumenten-ID | 53190 |
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