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Siday, Tom ; Sandner, Fabian ; Brem, Samuel ; Zizlsperger, Martin ; Perea-Causín, Raül ; Schiegl, Felix ; Nerreter, Svenja ; Plankl, Markus ; Merkl, Philipp ; Mooshammer, Fabian ; Huber, Markus A. ; Malic, Ermin ; Huber, Rupert

Ultrafast Nanoscopy of High-Density Exciton Phases in WSe2

Siday, Tom , Sandner, Fabian, Brem, Samuel, Zizlsperger, Martin, Perea-Causín, Raül, Schiegl, Felix, Nerreter, Svenja, Plankl, Markus, Merkl, Philipp, Mooshammer, Fabian , Huber, Markus A. , Malic, Ermin und Huber, Rupert (2022) Ultrafast Nanoscopy of High-Density Exciton Phases in WSe2. Nano Letters 22, S. 2561-2568.

Veröffentlichungsdatum dieses Volltextes: 14 Nov 2022 09:47
Artikel
DOI zum Zitieren dieses Dokuments: 10.5283/epub.53190


Zusammenfassung

The density-driven transition of an exciton gas into an electron- hole plasma remains a compelling question in condensed matter physics. In two-dimensional transition metal dichalcogenides, strongly bound excitons can undergo this phase change after transient injection of electron-hole pairs. Unfortunately, unavoidable nanoscale inhomogeneity in these materials has impeded quantitative ...

The density-driven transition of an exciton gas into an electron- hole plasma remains a compelling question in condensed matter physics. In two-dimensional transition metal dichalcogenides, strongly bound excitons can undergo this phase change after transient injection of electron-hole pairs. Unfortunately, unavoidable nanoscale inhomogeneity in these materials has impeded quantitative investigation into this elusive transition. Here, we demonstrate how ultrafast polarization nanoscopy can capture the Mott transition through the density-dependent recombination dynamics of electron-hole pairs within a WSe2 homobilayer. For increasing carrier density, an initial monomolecular recombination of optically dark excitons transitions continuously into a bimolecular recombination of an unbound electron-hole plasma above 7 x 10(12) cm(-2). We resolve how the Mott transition modulates over nanometer length scales, directly evidencing the strong inhomogeneity in stacked monolayers. Our results demonstrate how ultrafast polarization nanoscopy could unveil the interplay of strong electronic correlations and interlayer coupling within a diverse range of stacked and twisted two-dimensional materials.



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  • [img] Siday, Tom , Sandner, Fabian, Brem, Samuel, Zizlsperger, Martin, Perea-Causín, Raül, Schiegl, Felix, Nerreter, Svenja, Plankl, Markus, Merkl, Philipp, Mooshammer, Fabian , Huber, Markus A. , Malic, Ermin und Huber, Rupert (2022) Ultrafast Nanoscopy of High-Density Exciton Phases in WSe2. Nano Letters 22, S. 2561-2568. [Gegenwärtig angezeigt]

Details

DokumentenartArtikel
Titel eines Journals oder einer ZeitschriftNano Letters
Verlag:AMER CHEMICAL SOC
Ort der Veröffentlichung:WASHINGTON
Band:22
Seitenbereich:S. 2561-2568
Datum14 Februar 2022
InstitutionenPhysik > Institut für Experimentelle und Angewandte Physik > Lehrstuhl Professor Huber > Arbeitsgruppe Rupert Huber
Identifikationsnummer
WertTyp
10.1021/acs.nanolett.1c04741DOI
Stichwörter / KeywordsMONOLAYER; Mott transition; exciton; ultrafast dynamics; near-field microscopy; terahertz; transition metal dichalcogenides
Dewey-Dezimal-Klassifikation500 Naturwissenschaften und Mathematik > 530 Physik
StatusVeröffentlicht
BegutachtetJa, diese Version wurde begutachtet
An der Universität Regensburg entstandenJa
URN der UB Regensburgurn:nbn:de:bvb:355-epub-531902
Dokumenten-ID53190

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