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Irreducible tensor analysis of sum- and difference-frequency generation in partially oriented samples

URN to cite this document:
urn:nbn:de:bvb:355-epub-54959
DOI to cite this document:
10.5283/epub.5495
Dick, Bernhard
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Date of publication of this fulltext: 05 Aug 2009 13:50


Abstract

The macroscopic nonlinear optical susceptibility c(2) for a system of partially oriented mols. is written as the ensemble av. of mol. hyperpolarizability tensors b. The orientational distribution of these mols. is described by a probability function expanded in Wigner matrices. For a rotationally invariant system, c(2) has 7 nonvanishing components, and a method is outlined to det. these by sum- ...

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