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Irreducible tensor analysis of sum- and difference-frequency generation in partially oriented samples

Dick, Bernhard (1985) Irreducible tensor analysis of sum- and difference-frequency generation in partially oriented samples. Chemical Physics 96 (2), pp. 199-215.

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The macroscopic nonlinear optical susceptibility c(2) for a system of partially oriented mols. is written as the ensemble av. of mol. hyperpolarizability tensors b. The orientational distribution of these mols. is described by a probability function expanded in Wigner matrices. For a rotationally invariant system, c(2) has 7 nonvanishing components, and a method is outlined to det. these by sum- ...


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Item type:Article
Additional Information (public):CAN 103:45489 73-10 Optical, Electron, and Mass Spectroscopy and Other Related Properties
Institutions:Chemistry and Pharmacy > Institut für Physikalische und Theoretische Chemie > Chair of Chemistry III - Physical Chemistry (Molecular Spectroscopy and Photochemistry) > Prof. Dr. Bernhard Dick
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Keywords:Laser radiation (difference- or sum-frequency generation of, in partially oriented samples, irreducible tensor anal. of); Optical nonlinear property (susceptibility, second-order, of partially oriented samples, sum- or difference-frequency generation in relation to); laser sum difference frequency generation; nonlinear second order optical susceptibility
Dewey Decimal Classification:500 Science > 540 Chemistry & allied sciences
Refereed:Yes, this version has been refereed
Created at the University of Regensburg:No
Item ID:5495
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