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Response function theory of time-resolved CARS and CSRS of rotating molecules in liquids under general polarization conditions

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Dick, Bernhard
Date of publication of this fulltext: 05 Aug 2009 13:50


A theor. treatment of time-resolved CARS and CSRS is given that includes mol. rotation during the time interval between the excitation and probing light pulses. A mol. response function tensor was found that accounts for the vibrational relaxation and the rotational diffusion of the mols. The ensemble av. of this response function with an arbitrary set of polarization conditions for the light ...


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