Response functions and susceptibilities for multiresonant non-linear optical spectroscopy: perturbative computer algebra solution including feeding

URN to cite this document:: urn:nbn:de:bvb:355-epub-55031
DOI to cite this document:: 10.5283/epub.5503

Dick, Bernhard

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Date of publication of this fulltext: 05 Aug 2009 13:50

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Abstract

A diagrammatic perturbation theory is presented which permits the calcn. of a mol. non-linear-optical response function for a particular time sequence of light pulses, or a mol. non-linear-optical susceptibility for a particular combination of frequencies of the input light fields. Mol. relaxation is treated in the Markov approxn. The method also accounts for incoherent population transfer ...