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Dick, Bernhard

Response functions and susceptibilities for multiresonant non-linear optical spectroscopy: perturbative computer algebra solution including feeding

Dick, Bernhard (1993) Response functions and susceptibilities for multiresonant non-linear optical spectroscopy: perturbative computer algebra solution including feeding. Chemical Physics 171 (1-2), S. 59-78.

Veröffentlichungsdatum dieses Volltextes: 05 Aug 2009 13:50
Artikel
DOI zum Zitieren dieses Dokuments: 10.5283/epub.5503


Zusammenfassung

A diagrammatic perturbation theory is presented which permits the calcn. of a mol. non-linear-optical response function for a particular time sequence of light pulses, or a mol. non-linear-optical susceptibility for a particular combination of frequencies of the input light fields. Mol. relaxation is treated in the Markov approxn. The method also accounts for incoherent population transfer ...

A diagrammatic perturbation theory is presented which permits the calcn. of a mol. non-linear-optical response function for a particular time sequence of light pulses, or a mol. non-linear-optical susceptibility for a particular combination of frequencies of the input light fields. Mol. relaxation is treated in the Markov approxn. The method also accounts for incoherent population transfer between mol. levels as long as a hierarchical level ordering is possible. The diagrams are esp. useful for the selective generation of terms contg. a particular resonance of interest, or obeying the rotating wave approxn. The algorithm has been implemented in the symbolic algebra language REDUCE. These procedures allow the automatic generation of all diagrams evolving from a particular exptl. situation, and the automatic calcn. of the corresponding response function or susceptibility.



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Details

DokumentenartArtikel
Titel eines Journals oder einer ZeitschriftChemical Physics
Verlag:Elsevier
Band:171
Nummer des Zeitschriftenheftes oder des Kapitels:1-2
Seitenbereich:S. 59-78
Datum1993
Zusätzliche Informationen (Öffentlich)CAN 118:243936 73-10 Optical, Electron, and Mass Spectroscopy and Other Related Properties
InstitutionenChemie und Pharmazie > Institut für Physikalische und Theoretische Chemie > Chair of Chemistry III - Physical Chemistry (Molecular Spectroscopy and Photochemistry) > Prof. Dr. Bernhard Dick
Identifikationsnummer
WertTyp
1993:243936Andere
10.1016/0301-0104(93)85131-QDOI
Stichwörter / KeywordsAlgorithm (for response functions and susceptibilities for multiresonant nonlinear optical spectroscopy) Spectrometry Ultraviolet and visible spectrometry (nonlinear, response functions in susceptibilities for multiresonant) Optical nonlinear property (spectroscopy, response functions and susceptibility for multiresonant) Mathematics Quantum chemistry (perturbation theory, for response functions and susceptibilities for multiresonant nonlinear optical spectroscopy) perturbation theory multiresonant nonlinear optical spectroscopy
Dewey-Dezimal-Klassifikation500 Naturwissenschaften und Mathematik > 540 Chemie
StatusVeröffentlicht
BegutachtetJa, diese Version wurde begutachtet
An der Universität Regensburg entstandenJa
URN der UB Regensburgurn:nbn:de:bvb:355-epub-55031
Dokumenten-ID5503

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