| Download ( PDF | 1MB) |
Resonant nonlinear spectroscopy in strong fields
Dick, Bernhard und Hochstrasser, R. M. (1983) Resonant nonlinear spectroscopy in strong fields. Chemical Physics 75 (2), S. 133-155.Veröffentlichungsdatum dieses Volltextes: 05 Aug 2009 13:50
Artikel
DOI zum Zitieren dieses Dokuments: 10.5283/epub.5515
Zusammenfassung
A method is presented to describe multiple resonant nonlinear spectra in the presence of strong laser fields. The Liouville equation for the d. operator of the mol. system is transformed to a time-independent linear equation system. This can be easily solved rigorously by numerical methods or, after partitioning into a strong-field part and a perturbation, the soln. can be obtained anal. by a ...
A method is presented to describe multiple resonant nonlinear spectra in the presence of strong laser fields. The Liouville equation for the d. operator of the mol. system is transformed to a time-independent linear equation system. This can be easily solved rigorously by numerical methods or, after partitioning into a strong-field part and a perturbation, the soln. can be obtained anal. by a novel perturbative approach. The results account for power broadening. Rabi splitting of signals, and power-induced extra resonances, the latter being related to the pure dephasing-induced resonances in the weak-field limit. The method can be applied to a large no. of multiple resonant nonlinear spectroscopies, esp. CARS, CSRS, coherent Rayleigh scattering and sum- or difference-frequency generation.
Alternative Links zum Volltext
Beteiligte Einrichtungen
Details
| Dokumentenart | Artikel | ||||||
| Titel eines Journals oder einer Zeitschrift | Chemical Physics | ||||||
| Verlag: | Elsevier | ||||||
|---|---|---|---|---|---|---|---|
| Band: | 75 | ||||||
| Nummer des Zeitschriftenheftes oder des Kapitels: | 2 | ||||||
| Seitenbereich: | S. 133-155 | ||||||
| Datum | 1983 | ||||||
| Zusätzliche Informationen (Öffentlich) | CAN 98:152579 73-10 Optical, Electron, and Mass Spectroscopy and Other Related Properties | ||||||
| Institutionen | Chemie und Pharmazie > Institut für Physikalische und Theoretische Chemie > Chair of Chemistry III - Physical Chemistry (Molecular Spectroscopy and Photochemistry) > Prof. Dr. Bernhard Dick | ||||||
| Identifikationsnummer |
| ||||||
| Stichwörter / Keywords | Laser radiation (resonance nonlinear spectroscopy in strong fields of); Raman spectrometry (resonance nonlinear, in strong laser fields); Optical nonlinear property (resonance spectroscopy, in strong laser fields); Spectrometry (nonlinear, resonance, in strong laser fields); resonant nonlinear spectroscopy laser field | ||||||
| Dewey-Dezimal-Klassifikation | 500 Naturwissenschaften und Mathematik > 540 Chemie | ||||||
| Status | Veröffentlicht | ||||||
| Begutachtet | Ja, diese Version wurde begutachtet | ||||||
| An der Universität Regensburg entstanden | Nein | ||||||
| URN der UB Regensburg | urn:nbn:de:bvb:355-epub-55152 | ||||||
| Dokumenten-ID | 5515 |
Downloadstatistik
Downloadstatistik