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Dick, Bernhard ; Hochstrasser, R. M.

Resonant nonlinear spectroscopy in strong fields

Dick, Bernhard und Hochstrasser, R. M. (1983) Resonant nonlinear spectroscopy in strong fields. Chemical Physics 75 (2), S. 133-155.

Veröffentlichungsdatum dieses Volltextes: 05 Aug 2009 13:50
Artikel
DOI zum Zitieren dieses Dokuments: 10.5283/epub.5515


Zusammenfassung

A method is presented to describe multiple resonant nonlinear spectra in the presence of strong laser fields. The Liouville equation for the d. operator of the mol. system is transformed to a time-independent linear equation system. This can be easily solved rigorously by numerical methods or, after partitioning into a strong-field part and a perturbation, the soln. can be obtained anal. by a ...

A method is presented to describe multiple resonant nonlinear spectra in the presence of strong laser fields. The Liouville equation for the d. operator of the mol. system is transformed to a time-independent linear equation system. This can be easily solved rigorously by numerical methods or, after partitioning into a strong-field part and a perturbation, the soln. can be obtained anal. by a novel perturbative approach. The results account for power broadening. Rabi splitting of signals, and power-induced extra resonances, the latter being related to the pure dephasing-induced resonances in the weak-field limit. The method can be applied to a large no. of multiple resonant nonlinear spectroscopies, esp. CARS, CSRS, coherent Rayleigh scattering and sum- or difference-frequency generation.



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Details

DokumentenartArtikel
Titel eines Journals oder einer ZeitschriftChemical Physics
Verlag:Elsevier
Band:75
Nummer des Zeitschriftenheftes oder des Kapitels:2
Seitenbereich:S. 133-155
Datum1983
Zusätzliche Informationen (Öffentlich)CAN 98:152579 73-10 Optical, Electron, and Mass Spectroscopy and Other Related Properties
InstitutionenChemie und Pharmazie > Institut für Physikalische und Theoretische Chemie > Chair of Chemistry III - Physical Chemistry (Molecular Spectroscopy and Photochemistry) > Prof. Dr. Bernhard Dick
Identifikationsnummer
WertTyp
1983:152579Andere
10.1016/0301-0104(83)85015-0DOI
Stichwörter / KeywordsLaser radiation (resonance nonlinear spectroscopy in strong fields of); Raman spectrometry (resonance nonlinear, in strong laser fields); Optical nonlinear property (resonance spectroscopy, in strong laser fields); Spectrometry (nonlinear, resonance, in strong laser fields); resonant nonlinear spectroscopy laser field
Dewey-Dezimal-Klassifikation500 Naturwissenschaften und Mathematik > 540 Chemie
StatusVeröffentlicht
BegutachtetJa, diese Version wurde begutachtet
An der Universität Regensburg entstandenNein
URN der UB Regensburgurn:nbn:de:bvb:355-epub-55152
Dokumenten-ID5515

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