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Silver‐Catalyzed Enantioselective Sulfimidation Mediated by Hydrogen Bonding Interactions

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Annapureddy, Rajasekar Reddy ; Burg, Finn ; Gramüller, Johannes ; Golub, Tino P. ; Merten, Christian ; Huber, Stefan M. ; Bach, Thorsten
Date of publication of this fulltext: 29 Feb 2024 12:28


An enantioselective sulfimidation of 3-thiosubstituted 2-quinolones and 2-pyridones was achieved with a stoichiometric nitrene source (PhI=NNs) and a silver-based catalyst system. Key to the success of the reaction is the use of a chiral phenanthroline ligand with a hydrogen bonding site. The enantioselectivity does not depend on the size of the two substituents at the sulfur atom but only on the ...


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