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Chirality-controlled spin scattering through quantum interference
van Ruitenbeek, Jan M.
, Korytár, Richard und Evers, Ferdinand
(2023)
Chirality-controlled spin scattering through quantum interference.
The Journal of Chemical Physics 159 (2), 024710.
Veröffentlichungsdatum dieses Volltextes: 23 Apr 2024 08:13
Artikel
DOI zum Zitieren dieses Dokuments: 10.5283/epub.58130
Zusammenfassung
Chirality-induced spin selectivity has been reported in many experiments, but a generally accepted theoretical explanation has not yet been proposed. Here, we introduce a simple model system of a straight cylindrical free-electron wire containing a helical string of atomic scattering centers with spin-orbit interaction. The advantage of this simple model is that it allows deriving analytical ...
Chirality-induced spin selectivity has been reported in many experiments, but a generally accepted theoretical explanation has not yet been proposed. Here, we introduce a simple model system of a straight cylindrical free-electron wire containing a helical string of atomic scattering centers with spin-orbit interaction. The advantage of this simple model is that it allows deriving analytical expressions for the spin scattering rates, such that the origin of the effect can be easily followed. We find that spin-selective scattering can be viewed as resulting from the constructive interference of partial waves scattered by the spin-orbit terms. We demonstrate that forward scattering rates are independent of spin, while back scattering is spin dependent over wide windows of energy. Although the model does not represent the full details of electron transmission through chiral molecules, it clearly reveals a mechanism that could operate in chiral systems.
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| Dokumentenart | Artikel | ||||||
| Titel eines Journals oder einer Zeitschrift | The Journal of Chemical Physics | ||||||
| Verlag: | AIP Publishing | ||||||
|---|---|---|---|---|---|---|---|
| Ort der Veröffentlichung: | MELVILLE | ||||||
| Band: | 159 | ||||||
| Nummer des Zeitschriftenheftes oder des Kapitels: | 2 | ||||||
| Seitenbereich: | 024710 | ||||||
| Datum | 13 Juli 2023 | ||||||
| Institutionen | Physik > Institut für Theoretische Physik > Lehrstuhl Ferdinand Evers | ||||||
| Identifikationsnummer |
| ||||||
| Stichwörter / Keywords | DEPENDENT ELECTRON TRANSMISSION; MOLECULES; SELECTIVITY; | ||||||
| Dewey-Dezimal-Klassifikation | 500 Naturwissenschaften und Mathematik > 530 Physik 500 Naturwissenschaften und Mathematik > 540 Chemie | ||||||
| Status | Veröffentlicht | ||||||
| Begutachtet | Ja, diese Version wurde begutachtet | ||||||
| An der Universität Regensburg entstanden | Ja | ||||||
| URN der UB Regensburg | urn:nbn:de:bvb:355-epub-581306 | ||||||
| Dokumenten-ID | 58130 |
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