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Meineke, Christian ; Schlosser, Jakob ; Zizlsperger, Martin ; Liebich, Marlene ; Nilforoushan, Niloufar ; Mosina, Kseniia ; Terres, Sophia ; Chernikov, Alexey ; Sofer, Zdenek ; Huber, Markus A. ; Florian, Matthias ; Kira, Mackillo ; Dirnberger, Florian ; Huber, Rupert

Ultrafast Exciton Dynamics in the Atomically Thin van der Waals Magnet CrSBr

Meineke, Christian , Schlosser, Jakob, Zizlsperger, Martin, Liebich, Marlene, Nilforoushan, Niloufar, Mosina, Kseniia, Terres, Sophia, Chernikov, Alexey, Sofer, Zdenek, Huber, Markus A. , Florian, Matthias, Kira, Mackillo, Dirnberger, Florian and Huber, Rupert (2024) Ultrafast Exciton Dynamics in the Atomically Thin van der Waals Magnet CrSBr. Nano Letters 24 (14), pp. 4101-4107.

Date of publication of this fulltext: 17 May 2024 16:16
Article
DOI to cite this document: 10.5283/epub.58287


Abstract

Among atomically thin semiconductors, CrSBr stands out as both its bulk and monolayer forms host tightly bound, quasi-one-dimensional excitons in a magnetic environment. Despite its pivotal importance for solid-state research, the exciton lifetime has remained unknown. While terahertz polarization probing can directly trace all excitons, independently of interband selection rules, the ...

Among atomically thin semiconductors, CrSBr stands out as both its bulk and monolayer forms host tightly bound, quasi-one-dimensional excitons in a magnetic environment. Despite its pivotal importance for solid-state research, the exciton lifetime has remained unknown. While terahertz polarization probing can directly trace all excitons, independently of interband selection rules, the corresponding large far-field foci substantially exceed the lateral sample dimensions. Here, we combine terahertz polarization spectroscopy with near-field microscopy to reveal a femtosecond decay of paramagnetic excitons in a monolayer of CrSBr, which is 30 times shorter than the bulk lifetime. We unveil low-energy fingerprints of bound and unbound electron–hole pairs in bulk CrSBr and extract the nonequilibrium dielectric function of the monolayer in a model-free manner. Our results demonstrate the first direct access to the ultrafast dielectric response of quasi-one-dimensional excitons in CrSBr, potentially advancing the development of quantum devices based on ultrathin van der Waals magnets.



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  • [img] Meineke, Christian , Schlosser, Jakob, Zizlsperger, Martin, Liebich, Marlene, Nilforoushan, Niloufar, Mosina, Kseniia, Terres, Sophia, Chernikov, Alexey, Sofer, Zdenek, Huber, Markus A. , Florian, Matthias, Kira, Mackillo, Dirnberger, Florian and Huber, Rupert (2024) Ultrafast Exciton Dynamics in the Atomically Thin van der Waals Magnet CrSBr. Nano Letters 24 (14), pp. 4101-4107. [Currently displayed]

Details

Item typeArticle
Journal or Publication TitleNano Letters
Publisher:American Chemical Society (ACS)
Volume:24
Number of Issue or Book Chapter:14
Page Range:pp. 4101-4107
Date20 March 2024
InstitutionsPhysics > Institute of Experimental and Applied Physics
Physics > Institute of Experimental and Applied Physics > Chair Professor Huber > Group Rupert Huber
Projects
Funded by: Deutsche Forschungsgemeinschaft (DFG) (314695032)
Funded by: Deutsche Forschungsgemeinschaft (DFG) (UNSPECIFIED)
Identification Number
ValueType
10.1021/acs.nanolett.3c05010DOI
Keywordsatomically thin solids, van der Waals magnets, anisotropic excitons, ultrafast dynamics, femtosecond near-field microscopy, terahertz
Dewey Decimal Classification500 Science > 530 Physics
StatusPublished
RefereedYes, this version has been refereed
Created at the University of RegensburgYes
URN of the UB Regensburgurn:nbn:de:bvb:355-epub-582871
Item ID58287

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