| Veröffentlichte Version Download ( PDF | 3MB) | Lizenz: Creative Commons Namensnennung 4.0 International |
Ultrafast Exciton Dynamics in the Atomically Thin van der Waals Magnet CrSBr
Meineke, Christian
, Schlosser, Jakob, Zizlsperger, Martin, Liebich, Marlene, Nilforoushan, Niloufar, Mosina, Kseniia, Terres, Sophia, Chernikov, Alexey, Sofer, Zdenek, Huber, Markus A.
, Florian, Matthias, Kira, Mackillo, Dirnberger, Florian
und Huber, Rupert
(2024)
Ultrafast Exciton Dynamics in the Atomically Thin van der Waals Magnet CrSBr.
Nano Letters 24 (14), S. 4101-4107.
Veröffentlichungsdatum dieses Volltextes: 17 Mai 2024 16:16
Artikel
DOI zum Zitieren dieses Dokuments: 10.5283/epub.58287
Zusammenfassung
Among atomically thin semiconductors, CrSBr stands out as both its bulk and monolayer forms host tightly bound, quasi-one-dimensional excitons in a magnetic environment. Despite its pivotal importance for solid-state research, the exciton lifetime has remained unknown. While terahertz polarization probing can directly trace all excitons, independently of interband selection rules, the ...
Among atomically thin semiconductors, CrSBr stands out as both its bulk and monolayer forms host tightly bound, quasi-one-dimensional excitons in a magnetic environment. Despite its pivotal importance for solid-state research, the exciton lifetime has remained unknown. While terahertz polarization probing can directly trace all excitons, independently of interband selection rules, the corresponding large far-field foci substantially exceed the lateral sample dimensions. Here, we combine terahertz polarization spectroscopy with near-field microscopy to reveal a femtosecond decay of paramagnetic excitons in a monolayer of CrSBr, which is 30 times shorter than the bulk lifetime. We unveil low-energy fingerprints of bound and unbound electron–hole pairs in bulk CrSBr and extract the nonequilibrium dielectric function of the monolayer in a model-free manner. Our results demonstrate the first direct access to the ultrafast dielectric response of quasi-one-dimensional excitons in CrSBr, potentially advancing the development of quantum devices based on ultrathin van der Waals magnets.
Alternative Links zum Volltext
Beteiligte Einrichtungen
Verknüpfung von Datensätzen
-
Meineke, Christian
, Schlosser, Jakob, Zizlsperger, Martin, Liebich, Marlene, Nilforoushan, Niloufar, Mosina, Kseniia, Terres, Sophia, Chernikov, Alexey, Sofer, Zdenek, Huber, Markus A.
, Florian, Matthias, Kira, Mackillo, Dirnberger, Florian
und Huber, Rupert
(2024)
Ultrafast Exciton Dynamics in the Atomically Thin van der Waals Magnet CrSBr.
Nano Letters 24 (14), S. 4101-4107.
[Gegenwärtig angezeigt]-
Meineke, Christian
, Schlosser, Jakob, Zizlsperger, Martin
, Liebich, Marlene
, Nilforoushan, Niloufar
, Mosina, Kseniia, Terres, Sophia, Chernikov, Alexey, Sofer, Zdeněk, Huber, Markus A.
, Florian, Matthias, Kira, M., Dirnberger, Florian
und Huber, Rupert
(2024)
Data archive of 'Ultrafast Exciton Dynamics in the Atomically Thin van der Waals Magnet CrSBr'.
[Datensatz]
-
Meineke, Christian
, Schlosser, Jakob, Zizlsperger, Martin
, Liebich, Marlene, Nilforoushan, Niloufar
, Mosina, Kseniia, Terres, Sophia, Chernikov, Alexey, Sofer, Zdenek
, Huber, Markus A.
, Florian, Matthias, Kira, Mackillo, Dirnberger, Florian
und Huber, Rupert
(2025)
Data Archive of "Ultrafast Exciton Dynamics in the Atomically Thin van der Waals Magnet CrSBr ".
[Datensatz]
-
Details
| Dokumentenart | Artikel | ||||
| Titel eines Journals oder einer Zeitschrift | Nano Letters | ||||
| Verlag: | American Chemical Society (ACS) | ||||
|---|---|---|---|---|---|
| Band: | 24 | ||||
| Nummer des Zeitschriftenheftes oder des Kapitels: | 14 | ||||
| Seitenbereich: | S. 4101-4107 | ||||
| Datum | 20 März 2024 | ||||
| Institutionen | Physik > Institut für Experimentelle und Angewandte Physik Physik > Institut für Experimentelle und Angewandte Physik > Lehrstuhl Professor Huber > Arbeitsgruppe Rupert Huber | ||||
| Projekte |
Gefördert von:
Deutsche Forschungsgemeinschaft (DFG)
(314695032)
Gefördert von:
Deutsche Forschungsgemeinschaft (DFG)
(Nicht ausgewählt)
| ||||
| Identifikationsnummer |
| ||||
| Stichwörter / Keywords | atomically thin solids, van der Waals magnets, anisotropic excitons, ultrafast dynamics, femtosecond near-field microscopy, terahertz | ||||
| Dewey-Dezimal-Klassifikation | 500 Naturwissenschaften und Mathematik > 530 Physik | ||||
| Status | Veröffentlicht | ||||
| Begutachtet | Ja, diese Version wurde begutachtet | ||||
| An der Universität Regensburg entstanden | Ja | ||||
| URN der UB Regensburg | urn:nbn:de:bvb:355-epub-582871 | ||||
| Dokumenten-ID | 58287 |
Downloadstatistik
Downloadstatistik