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Ultrafast Exciton Dynamics in the Atomically Thin van der Waals Magnet CrSBr

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Meineke, Christian ; Schlosser, Jakob ; Zizlsperger, Martin ; Liebich, Marlene ; Nilforoushan, Niloufar ; Mosina, Kseniia ; Terres, Sophia ; Chernikov, Alexey ; Sofer, Zdenek ; Huber, Markus A. ; Florian, Matthias ; Kira, Mackillo ; Dirnberger, Florian ; Huber, Rupert
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Date of publication of this fulltext: 17 May 2024 16:16


Among atomically thin semiconductors, CrSBr stands out as both its bulk and monolayer forms host tightly bound, quasi-one-dimensional excitons in a magnetic environment. Despite its pivotal importance for solid-state research, the exciton lifetime has remained unknown. While terahertz polarization probing can directly trace all excitons, independently of interband selection rules, the ...


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