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Design, Synthesis, and Evaluation of a Biomimetic Artificial Photolyase Model

Wiest, O. ; Harrison, C. B. ; Saettel, N. J. ; Cibulka, R. ; Sax, M. ; König, B.


Two new artificial photolyase models that recognize pyrimidine dimers in protic and aprotic organic solvents as well as in water through a combination of charge and hydrogen-bonding interactions and use a mimic of the flavine to achieve repair through reductive photoinduced electron transfer are presented. Fluorescence and NMR titration studies show that it forms a 1:1 complex with pyrimidine ...


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