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Generalized many-body exciton g-factors: magnetic hybridization and non-monotonic Rydberg series in monolayer WSe2
Paulo Eduardo, de Faria Junior
(2025)
Generalized many-body exciton g-factors: magnetic hybridization and non-monotonic Rydberg series in monolayer WSe2.
arXiv.
(In Press)
Date of publication of this fulltext: 12 Nov 2025 15:46
Article
DOI to cite this document: 10.5283/epub.78132
Abstract
Magneto-optics of low dimensional semiconductors, such as monolayer transition metal dichalcogenides, offers a vast playground for exploring complex quantum phenomena. However, current ab initio approaches fail to capture important experimental observations related to brightening of excitonic levels and their g-factor dependence. Here, we develop a robust and general first principles framework ...
Magneto-optics of low dimensional semiconductors, such as monolayer transition metal dichalcogenides, offers a vast playground for exploring complex quantum phenomena. However, current ab initio approaches fail to capture important experimental observations related to brightening of excitonic levels and their g-factor dependence. Here, we develop a robust and general first principles framework for many-body exciton g-factors by incorporating off-diagonal terms for the spin and orbital angular momenta of single-particle bands and many-body states for magnetic fields pointing in arbitrary spatial directions. We implement our framework using many-body perturbation theory via the GW-Bethe-Salpeter equation (BSE) and supplement our analysis with robust symmetry-based models, establishing a fruitful synergy between many-body GW-BSE and group theory. Focusing on the archetypal monolayer WSe_2, we accurately reproduce the known results of the low-energy excitons including the Zeeman splitting and the dark/grey exciton brightening. Furthermore, our theory naturally reveals fundamental physical mechanisms of magnetic-field hybridization of higher-energy excitons (s- and p-like) and resolves the long-standing puzzle of the experimentally measured non-monotonic Rydberg series (1s-4s) of exciton g-factors. Our framework offers a comprehensive approach to investigate, rationalize, and predict the non-trivial interplay between magnetic fields, angular momenta, and many-body exciton physics in van der Waals systems.
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Paulo Eduardo, de Faria Junior
(2025)
Generalized many-body exciton g-factors: magnetic hybridization and non-monotonic Rydberg series in monolayer WSe2.
arXiv.
(In Press)
[Currently displayed]-
Faria Junior, Paulo E.
, Hernangómez-Pérez, Daniel
, Amit, Tomer
, Fabian, Jaroslav
and Refaely-Abramson, Sivan
(2025)
Generalized many-body exciton g factors: Magnetic hybridization and nonmonotonic Rydberg series in monolayer WSe₂.
Physical Review B 112, L241404.
-
Details
| Item type | Article | ||||
| Journal or Publication Title | arXiv | ||||
| Open Access Type: | OA-Version in anderem Repositorium | ||||
|---|---|---|---|---|---|
| Date | 2 June 2025 | ||||
| Institutions | Physics > Institute of Theroretical Physics > Chair Professor Richter > Group Jaroslav Fabian | ||||
| Projects |
Funded by:
Deutsche Forschungsgemeinschaft (DFG)
(314695032)
| ||||
| Identification Number |
| ||||
| Keywords | Subjects: Mesoscale and Nanoscale Physics (cond-mat.mes-hall); Materials Science (cond-mat.mtrl-sci) | ||||
| Dewey Decimal Classification | 500 Science > 530 Physics | ||||
| Status | In Press | ||||
| Refereed | Yes, this version has been refereed | ||||
| Created at the University of Regensburg | Yes | ||||
| URN of the UB Regensburg | urn:nbn:de:bvb:355-epub-781329 | ||||
| Item ID | 78132 |
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