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Generalized many-body exciton g factors: Magnetic hybridization and nonmonotonic Rydberg series in monolayer WSe₂
Faria Junior, Paulo E.
, Hernangómez-Pérez, Daniel
, Amit, Tomer
, Fabian, Jaroslav
und Refaely-Abramson, Sivan
(2025)
Generalized many-body exciton g factors: Magnetic hybridization and nonmonotonic Rydberg series in monolayer WSe₂.
Physical Review B 112, L241404.
Veröffentlichungsdatum dieses Volltextes: 10 Dez 2025 10:51
Artikel
DOI zum Zitieren dieses Dokuments: 10.5283/epub.78313
Zusammenfassung
The magneto-optical response of excitons in monolayer transition metal dichalcogenides is governed by a complex interplay of Bloch-state quantum geometry—reflected in the electronic magnetic moment—coupled with interband mixing and many-body interactions. Here, we develop a robust and general first-principles framework for many-body exciton g factors (magnetic moments) by incorporating ...
The magneto-optical response of excitons in monolayer transition metal dichalcogenides is governed by a complex interplay of Bloch-state quantum geometry—reflected in the electronic magnetic moment—coupled with interband mixing and many-body interactions. Here, we develop a robust and general first-principles framework for many-body exciton g factors (magnetic moments) by incorporating off-diagonal terms for the spin and orbital angular momenta of single-particle bands and many-body states for magnetic fields pointing in arbitrary spatial directions. We implement our framework using many-body perturbation theory via the GW-Bethe-Salpeter equation and supplement our analysis with robust symmetry-based models. Focusing on the archetypal monolayer WSe₂, we accurately reproduce the known results of the low-energy excitons including the Zeeman splitting and the dark/gray exciton brightening. Furthermore, our theory naturally reveals the magnetic-field hybridization of higher-energy excitons (s, p, and d like) and shows that the magnetic moments of nodal excitons (p and d like) do not acquire additional contributions of ±mⱼµB (mⱼ=1,2), characteristic of the hydrogenic picture. Our general approach also allows us to resolve the long-standing puzzle of the experimentally measured nonmonotonic Rydberg series (1s−4s) of exciton g factors. Our framework offers a comprehensive approach to investigate, rationalize, and predict the nontrivial interplay between magnetic fields, angular momenta, and many-body exciton physics in van der Waals systems, offering different opportunities to probe signatures of quantum geometry within many-body states.
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Beteiligte Einrichtungen
Verknüpfung von Datensätzen
-
Paulo Eduardo, de Faria Junior
(2025)
Generalized many-body exciton g-factors: magnetic hybridization and non-monotonic Rydberg series in monolayer WSe2.
arXiv.
(Im Druck)
Details
| Dokumentenart | Artikel | ||||
| Titel eines Journals oder einer Zeitschrift | Physical Review B | ||||
| Verlag: | American Physical Society (APS) | ||||
|---|---|---|---|---|---|
| Band: | 112 | ||||
| Seitenbereich: | L241404 | ||||
| Datum | 3 Dezember 2025 | ||||
| Institutionen | Physik > Institut für Theoretische Physik > Lehrstuhl Professor Richter > Arbeitsgruppe Jaroslav Fabian | ||||
| Projekte |
Gefördert von:
Deutsche Forschungsgemeinschaft (DFG)
(314695032)
| ||||
| Identifikationsnummer |
| ||||
| Stichwörter / Keywords | Bethe-Salpeter equation Excitons Magneto-optics Spin-orbit coupling Transition metal dichalcogenides Group theory | ||||
| Dewey-Dezimal-Klassifikation | 500 Naturwissenschaften und Mathematik > 530 Physik | ||||
| Status | Veröffentlicht | ||||
| Begutachtet | Ja, diese Version wurde begutachtet | ||||
| An der Universität Regensburg entstanden | Zum Teil | ||||
| URN der UB Regensburg | urn:nbn:de:bvb:355-epub-783131 | ||||
| Dokumenten-ID | 78313 |
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