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Faria Junior, Paulo E. ; Hernangómez-Pérez, Daniel ; Amit, Tomer ; Fabian, Jaroslav ; Refaely-Abramson, Sivan

Generalized many-body exciton g factors: Magnetic hybridization and nonmonotonic Rydberg series in monolayer WSe₂

Faria Junior, Paulo E. , Hernangómez-Pérez, Daniel , Amit, Tomer , Fabian, Jaroslav und Refaely-Abramson, Sivan (2025) Generalized many-body exciton g factors: Magnetic hybridization and nonmonotonic Rydberg series in monolayer WSe₂. Physical Review B 112, L241404.

Veröffentlichungsdatum dieses Volltextes: 10 Dez 2025 10:51
Artikel
DOI zum Zitieren dieses Dokuments: 10.5283/epub.78313


Zusammenfassung

The magneto-optical response of excitons in monolayer transition metal dichalcogenides is governed by a complex interplay of Bloch-state quantum geometry—reflected in the electronic magnetic moment—coupled with interband mixing and many-body interactions. Here, we develop a robust and general first-principles framework for many-body exciton g factors (magnetic moments) by incorporating ...

The magneto-optical response of excitons in monolayer transition metal dichalcogenides is governed by a complex interplay of Bloch-state quantum geometry—reflected in the electronic magnetic moment—coupled with interband mixing and many-body interactions. Here, we develop a robust and general first-principles framework for many-body exciton g factors (magnetic moments) by incorporating off-diagonal terms for the spin and orbital angular momenta of single-particle bands and many-body states for magnetic fields pointing in arbitrary spatial directions. We implement our framework using many-body perturbation theory via the GW-Bethe-Salpeter equation and supplement our analysis with robust symmetry-based models. Focusing on the archetypal monolayer WSe₂, we accurately reproduce the known results of the low-energy excitons including the Zeeman splitting and the dark/gray exciton brightening. Furthermore, our theory naturally reveals the magnetic-field hybridization of higher-energy excitons (s, p, and d like) and shows that the magnetic moments of nodal excitons (p and d like) do not acquire additional contributions of ±mⱼ⁢µB (mⱼ=1,2), characteristic of the hydrogenic picture. Our general approach also allows us to resolve the long-standing puzzle of the experimentally measured nonmonotonic Rydberg series (1⁢s−4s) of exciton g factors. Our framework offers a comprehensive approach to investigate, rationalize, and predict the nontrivial interplay between magnetic fields, angular momenta, and many-body exciton physics in van der Waals systems, offering different opportunities to probe signatures of quantum geometry within many-body states.



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Details

DokumentenartArtikel
Titel eines Journals oder einer ZeitschriftPhysical Review B
Verlag:American Physical Society (APS)
Band:112
Seitenbereich:L241404
Datum3 Dezember 2025
InstitutionenPhysik > Institut für Theoretische Physik > Lehrstuhl Professor Richter > Arbeitsgruppe Jaroslav Fabian
Projekte
Gefördert von: Deutsche Forschungsgemeinschaft (DFG) (314695032)
Identifikationsnummer
WertTyp
10.1103/c5y7-w9tkDOI
Stichwörter / KeywordsBethe-Salpeter equation Excitons Magneto-optics Spin-orbit coupling Transition metal dichalcogenides Group theory
Dewey-Dezimal-Klassifikation500 Naturwissenschaften und Mathematik > 530 Physik
StatusVeröffentlicht
BegutachtetJa, diese Version wurde begutachtet
An der Universität Regensburg entstandenZum Teil
URN der UB Regensburgurn:nbn:de:bvb:355-epub-783131
Dokumenten-ID78313

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