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van Ruitenbeek, Jan M. ; Korytár, Richard ; Evers, Ferdinand

Chirality-controlled spin scattering through quantum interference

van Ruitenbeek, Jan M. , Korytár, Richard und Evers, Ferdinand (2023) Chirality-controlled spin scattering through quantum interference. The Journal of Chemical Physics 159 (2), 024710.

Veröffentlichungsdatum dieses Volltextes: 23 Apr 2024 08:13
Artikel
DOI zum Zitieren dieses Dokuments: 10.5283/epub.58130


Zusammenfassung

Chirality-induced spin selectivity has been reported in many experiments, but a generally accepted theoretical explanation has not yet been proposed. Here, we introduce a simple model system of a straight cylindrical free-electron wire containing a helical string of atomic scattering centers with spin-orbit interaction. The advantage of this simple model is that it allows deriving analytical ...

Chirality-induced spin selectivity has been reported in many experiments, but a generally accepted theoretical explanation has not yet been proposed. Here, we introduce a simple model system of a straight cylindrical free-electron wire containing a helical string of atomic scattering centers with spin-orbit interaction. The advantage of this simple model is that it allows deriving analytical expressions for the spin scattering rates, such that the origin of the effect can be easily followed. We find that spin-selective scattering can be viewed as resulting from the constructive interference of partial waves scattered by the spin-orbit terms. We demonstrate that forward scattering rates are independent of spin, while back scattering is spin dependent over wide windows of energy. Although the model does not represent the full details of electron transmission through chiral molecules, it clearly reveals a mechanism that could operate in chiral systems.



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Details

DokumentenartArtikel
Titel eines Journals oder einer ZeitschriftThe Journal of Chemical Physics
Verlag:AIP Publishing
Ort der Veröffentlichung:MELVILLE
Band:159
Nummer des Zeitschriftenheftes oder des Kapitels:2
Seitenbereich:024710
Datum13 Juli 2023
InstitutionenPhysik > Institut für Theoretische Physik > Lehrstuhl Ferdinand Evers
Identifikationsnummer
WertTyp
10.1063/5.0156316DOI
2307.06201arXiv-ID
Stichwörter / KeywordsDEPENDENT ELECTRON TRANSMISSION; MOLECULES; SELECTIVITY;
Dewey-Dezimal-Klassifikation500 Naturwissenschaften und Mathematik > 530 Physik
500 Naturwissenschaften und Mathematik > 540 Chemie
StatusVeröffentlicht
BegutachtetJa, diese Version wurde begutachtet
An der Universität Regensburg entstandenJa
URN der UB Regensburgurn:nbn:de:bvb:355-epub-581306
Dokumenten-ID58130

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