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Okobayashi, Norio ; Gustafsson, Alexander ; Peronio, Angelo ; Paulsson, Magnus ; Arai, Toyoko ; Giessibl, Franz J.

Influence of atomic tip structure on the intensity of inelastic tunneling spectroscopy data analyzed by combined scanning tunneling spectroscopy, force microscopy, and density functional theory

Okobayashi, Norio, Gustafsson, Alexander, Peronio, Angelo , Paulsson, Magnus, Arai, Toyoko und Giessibl, Franz J. (2016) Influence of atomic tip structure on the intensity of inelastic tunneling spectroscopy data analyzed by combined scanning tunneling spectroscopy, force microscopy, and density functional theory. Physical Review B (PRB) 93, S. 165415-1.

Veröffentlichungsdatum dieses Volltextes: 27 Mai 2016 05:37
Artikel
DOI zum Zitieren dieses Dokuments: 10.5283/epub.33799


Zusammenfassung

Achieving a high intensity in inelastic scanning tunneling spectroscopy (IETS) is important for precise measurements. The intensity of the IETS signal can vary by up to a factor of 3 for various tips without an apparent reason accessible by scanning tunneling microscopy (STM) alone. Here, we show that combining STM and IETS with atomic force microscopy enables carbon monoxide front-atom ...

Achieving a high intensity in inelastic scanning tunneling spectroscopy (IETS) is important for precise measurements. The intensity of the IETS signal can vary by up to a factor of 3 for various tips without an apparent reason accessible by scanning tunneling microscopy (STM) alone. Here, we show that combining STM and IETS with atomic force microscopy enables carbon monoxide front-atom identification, revealing that high IETS intensities for CO/Cu(111) are obtained for single-atom tips, while the intensity drops sharply for multiatom tips. Adsorption of the CO molecule on a Cu adatom [CO/Cu/Cu(111)] such that the molecule is elevated over the substrate strongly diminishes the tip dependence of IETS intensity, showing that an elevated position channels most of the tunneling current through the CO molecule even for multiatom tips, while a large fraction of the tunneling current bypasses the CO molecule in the case of CO/Cu(111).



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Details

DokumentenartArtikel
Titel eines Journals oder einer ZeitschriftPhysical Review B (PRB)
Verlag:AMER PHYSICAL SOC
Ort der Veröffentlichung:COLLEGE PK
Band:93
Seitenbereich:S. 165415-1
Datum13 April 2016
InstitutionenPhysik > Institut für Experimentelle und Angewandte Physik > Lehrstuhl Professor Giessibl > Arbeitsgruppe Franz J. Giessibl
Identifikationsnummer
WertTyp
10.1103/PhysRevB.93.165415DOI
Stichwörter / KeywordsMOLECULE VIBRATIONAL SPECTROSCOPY; RESOLUTION; CO;
Dewey-Dezimal-Klassifikation500 Naturwissenschaften und Mathematik > 530 Physik
StatusVeröffentlicht
BegutachtetJa, diese Version wurde begutachtet
An der Universität Regensburg entstandenZum Teil
URN der UB Regensburgurn:nbn:de:bvb:355-epub-337993
Dokumenten-ID33799

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