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Apparent Reversal of Molecular Orbitals Reveals Entanglement

Yu, Ping , Kocić, Nemanja, Repp, Jascha , Siegert, Benjamin and Donarini, Andrea (2017) Apparent Reversal of Molecular Orbitals Reveals Entanglement. Physical Review Letters 119 (5), 056801.

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Date of publication of this fulltext: 08 Aug 2017 05:56

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Other URL: http://doi.org/10.1103/PhysRevLett.119.056801


Abstract

The frontier orbital sequence of individual dicyanovinyl-substituted oligothiophene molecules is studied by means of scanning tunneling microscopy. On NaCl/Cud(111), the molecules are neutral, and the two lowest unoccupied molecular states are observed in the expected order of increasing energy. On NaCl/Cud(311), where the molecules are negatively charged, the sequence of two observed molecular ...

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Item type:Article
Date:1 August 2017
Institutions:Physics > Institute of Theroretical Physics > Chair Professor Grifoni > Group Milena Grifoni
Physics > Institute of Theroretical Physics > Chair Professor Grifoni > Group John Schliemann
Physics > Institute of Theroretical Physics > Chair Professor Grifoni > Group Ferdinand Evers
Physics > Institute of Theroretical Physics > Chair Professor Grifoni > Group David Egger
Physics > Institute of Experimental and Applied Physics > Chair Professor Giessibl > Group Jascha Repp
Projects:SFB 689: Spinphänomene in reduzierten Dimensionen, GRK 1570, Elektronische Eigenschaften von Nanostrukturen auf Kohlenstoff-Basis
Identification Number:
ValueType
10.1103/PhysRevLett.119.056801DOI
Keywords:ATOMIC-FORCE MICROSCOPY; PI-CONJUGATED MOLECULES; SINGLE-MOLECULE; ELECTRONIC-STRUCTURE; WORK FUNCTION; CHARGE-STATE; OLIGOTHIOPHENE; INTERFERENCE; CONDUCTANCE; WIRES;
Dewey Decimal Classification:500 Science > 530 Physics
Status:Published
Refereed:Yes, this version has been refereed
Created at the University of Regensburg:Yes
Item ID:36073
Owner only: item control page

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