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Selective Single C(sp3)−F Bond Cleavage in Trifluoromethylarenes: Merging Visible-Light Catalysis with Lewis Acid Activation

Chen, Kang ; Berg, Nele ; Gschwind, Ruth Maria ; König, Burkhard



Abstract

The conversion of easily available trifluoromethylarenes into aryldifluoromethyl compounds, which are valuable motifs in the pharmaceutical chemistry, is highly atom-and step-economical. However, the single C(sp(3))-F bond cleavage of ArCF3 is a great challenge because of the chemical inertness of the C(sp(3))-F bond and the difficult selectivity control of monodefluorination. We report here the ...

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