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Design of hydrogels for delayed antibody release utilizing hydrophobic association and Diels–Alder chemistry in tandem

Gregoritza, Manuel ; Messmann, Viktoria ; Goepferich, Achim M. ; Brandl, Ferdinand P.



Abstract

Biodegradable hydrogels were prepared from furan-and maleimide-functionalized eight-armed poly-(ethylene glycol) with an average molecular mass of 40000 Da (8armPEG40k-furan and 8armPEG40k-maleimide) using the Diels-Alder (DA) reaction as a cross-linking mechanism. Hydrophobic 6-aminohexanoic acid (C-6) and 12-aminododecanoic acid (C-12) spacers were introduced between the polymer backbone and ...

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